Stability Issues in Electrochemical CO2 Reduction: Recent Advances in Fundamental Understanding and Design Strategies

W Lai, Y Qiao, Y Wang, H Huang - Advanced Materials, 2023 - Wiley Online Library
Electrochemical CO2 reduction reaction (CO2RR) offers a promising approach to close the
anthropogenic carbon cycle and store intermittent renewable energy in fuels or chemicals …

Operando scanning electrochemical probe microscopy during electrocatalysis

C Santana Santos, BN Jaato, I Sanjuán… - Chemical …, 2023 - ACS Publications
Scanning electrochemical probe microscopy (SEPM) techniques can disclose the local
electrochemical reactivity of interfaces in single-entity and sub-entity studies. Operando …

Atomic-scale surface restructuring of copper electrodes under CO2 electroreduction conditions

R Amirbeigiarab, J Tian, A Herzog, C Qiu… - Nature Catalysis, 2023 - nature.com
Potentiodynamic methods that induce structural changes in Cu catalysts for the
electrochemical reduction of CO2 (CO2RR) have been identified as a promising strategy for …

The significance of properly reporting turnover frequency in electrocatalysis research

S Anantharaj, PE Karthik, S Noda - … Chemie International Edition, 2021 - Wiley Online Library
For decades, turnover frequency (TOF) has served as an accurate descriptor of the intrinsic
activity of a catalyst, including those in electrocatalytic reactions involving both fuel …

Tailoring the Surface and Interface Structures of Copper‐Based Catalysts for Electrochemical Reduction of CO2 to Ethylene and Ethanol

Z Zhang, L Bian, H Tian, Y Liu, Y Bando, Y Yamauchi… - Small, 2022 - Wiley Online Library
Electrochemical CO2 reduction to valuable ethylene and ethanol offers a promising strategy
to lower CO2 emissions while storing renewable electricity. Cu‐based catalysts have shown …

Modeling Operando Electrochemical CO2 Reduction

F Dattila, RR Seemakurthi, Y Zhou, N López - Chemical Reviews, 2022 - ACS Publications
Since the seminal works on the application of density functional theory and the
computational hydrogen electrode to electrochemical CO2 reduction (eCO2R) and …

Linking the Dynamic Chemical State of Catalysts with the Product Profile of Electrocatalytic CO2 Reduction

J Wang, HY Tan, Y Zhu, H Chu… - Angewandte Chemie, 2021 - Wiley Online Library
The promoted activity and enhanced selectivity of electrocatalysts is commonly ascribed to
specific structural features such as surface facets, morphology, and atomic defects …

Progress and Perspectives of Electrochemical CO2 Reduction on Copper in Aqueous Electrolyte

S Nitopi, E Bertheussen, SB Scott, X Liu… - Chemical …, 2019 - ACS Publications
To date, copper is the only heterogeneous catalyst that has shown a propensity to produce
valuable hydrocarbons and alcohols, such as ethylene and ethanol, from electrochemical …

The role of in situ generated morphological motifs and Cu(i) species in C2+ product selectivity during CO2 pulsed electroreduction

RM Arán-Ais, F Scholten, S Kunze, R Rizo… - Nature Energy, 2020 - nature.com
The efficient electrochemical conversion of CO2 provides a route to fuels and feedstocks.
Copper catalysts are well-known to be selective to multicarbon products, although the role …

Designing materials for electrochemical carbon dioxide recycling

MB Ross, P De Luna, Y Li, CT Dinh, D Kim, P Yang… - Nature Catalysis, 2019 - nature.com
Electrochemical carbon dioxide recycling provides an attractive approach to synthesizing
fuels and chemical feedstocks using renewable energy. On the path to deploying this …