Intelligent ion gels: Design, performance, and applications

N Gao, C Pan - SmartMat, 2024 - Wiley Online Library
Intelligent ion gels, which possess highly tunable mechanical, electrical, and stimulus‐
responsive properties, have emerged as powerful candidates in the field of artificial …

The promising application of hydrogel microneedles in medical application

Y Wu, Z Tang, S Ma, L Du - Journal of Pharmacy and …, 2023 - academic.oup.com
Objectives Hydrogel microneedles are emerging, and promising microneedles mainly
composed of swelling polymers. This review is intended to summarize the preparation …

Polyelectrolyte complex-covalent interpenetrating polymer network hydrogels

D Li, T Göckler, U Schepers, S Srivastava - Macromolecules, 2022 - ACS Publications
Polyelectrolyte complex (PEC) hydrogels possess rich microstructural diversity and tunability
of the shear response, self-healing attributes, and pH-and salt-responsiveness. Yet, their …

Multicompartment hydrogels

BVKJ Schmidt - Macromolecular Rapid Communications, 2022 - Wiley Online Library
Hydrogels belong to the most promising materials in polymer and materials science at the
moment. As they feature soft and tissue‐like character as well as high water‐content, a …

pH response of sequence-controlled polyampholyte brushes

X Yuan, HW Hatch, JC Conrad, AB Marciel, JC Palmer - Soft Matter, 2023 - pubs.rsc.org
We use molecular simulation to investigate the pH response of sequence-controlled
polyampholyte brushes (PABs) with polymer chains consisting of alternating blocks of …

Sequestration of Small Ions and Weak Acids and Bases by a Polyelectrolyte Complex Studied by Simulation and Experiment

R Stano, JJ van Lente, S Lindhoud… - Macromolecules, 2024 - ACS Publications
Mixing of oppositely charged polyelectrolytes can result in phase separation into a polymer-
poor supernatant and a polymer-rich polyelectrolyte complex (PEC). We present a new …

How Charge Regulation Affects pH-Responsive Ampholyte Uptake in Weak Polyelectrolyte Brushes

K Radhakrishnan, D Beyer, C Holm - Macromolecules, 2024 - ACS Publications
Weak polyelectrolyte brushes are a promising platform for the selective capture and release
of charged proteins from bulk solutions. Despite their potential for creating smart responsive …

Advances, Applications, and Emerging Opportunities in Electrostatic Hydrogels

H Senebandith, D Li, S Srivastava - Langmuir, 2023 - ACS Publications
Polyelectrolyte complex (PEC) hydrogels, which self-assemble via complexation of
oppositely charged block polymers, have recently risen to prominence owing to their unique …

The pH-dependent swelling of weak polyelectrolyte hydrogels modeled at different levels of resolution

J Landsgesell, D Beyer, P Hebbeker… - …, 2022 - ACS Publications
The swelling of polyelectrolyte hydrogels has been often explained using simple models
derived from the Flory–Rehner model. While these models qualitatively predict the …

Charge regulation triggers condensation of short oligopeptides to polyelectrolytes

SP Pineda, R Staňo, A Murmiliuk, PM Blanco… - JACS Au, 2024 - ACS Publications
Electrostatic interactions between charged macromolecules are ubiquitous in biological
systems, and they are important also in materials design. Attraction between oppositely …