Enhancement of nonlinear optical response of 26Adamanzane by doping with alkali metals exohedrally and alkaline earth metals endohedrally: a DFT study

R Akbar, A Asif, N Maqsood, M Nouman - Structural Chemistry, 2024 - Springer
The quest for nonlinear optical (NLO) crystals, which are essential for future optical
understanding, detailed evaluations, and present laser gadgets, is a prominent concern in …

Hyper-Rayleigh scattering in centrosymmetric systems

MD Williams, JS Ford, DL Andrews - The Journal of Chemical Physics, 2015 - pubs.aip.org
Hyper-Rayleigh scattering (HRS) is an incoherent mechanism for optical second harmonic
generation. The frequency-doubled light that emerges from this mechanism is not emitted in …

Assessing limitations to the two-level approximation in nonlinear optics for organic chromophores by ab initio methods

MM Coles, JN Peck, VS Oganesyan… - Linear and Nonlinear …, 2011 - spiedigitallibrary.org
The use of a two-level approximation to simply characterize the nonlinear optical properties
of organic materials is well known. Usually only electronic ground states are significantly …

Mechanisms universally permitting hyper-Rayleigh scattering

MD Williams, JS Ford… - … and Conversion: Materials …, 2015 - spiedigitallibrary.org
Hyper-Rayleigh scattering (HRS) is an incoherent variant of second harmonic generation.
The theory involves terms of increasing order of optical nonlinearity: for molecules or unit …

Failure of the two-level and sum over states methods in nonlinear optics, demonstrated by ab initio methods

MM Coles, JN Peck, VS Oganesyan… - Nonlinear Optics and …, 2012 - spiedigitallibrary.org
When calculating nonlinear susceptibilities, a widely used two-level approximation in a sum-
over states formulation is the exclusion of all but the ground state and one single excited …

A quantum electrodynamical approach to nonlinear and structured light interactions with matter

M Williams - 2016 - ueaeprints.uea.ac.uk
This thesis employs molecular quantum electrodynamical theory to analyse the interactions
between light and matter for four main processes. The first to be considered is Raman …

[PDF][PDF] A QED framework for nonlinear and singular optics

M Coles - 2014 - ueaeprints.uea.ac.uk
The theory of quantum electrodynamics is employed in the description of linear and
nonlinear optical effects. We study the effects of using a two energy level approximation in …