Although the importance of water interfaces has long been well recognized, studies of the
interfaces at the molecular level only began more recently. 1-3 The difficulty lies in the fact …

The investigation of structural and dynamical properties of weakly bound clusters has
attracted a great deal of interest in recent years. 1-5 They provide an exceptional tool to …

The ubiquitous nature of water makes the study of water both practical and relevant. Yet in
this advanced technological age, many important, fundamental questions remain …

The molecular structure of the interfacial regions of aqueous electrolytes is poorly
understood, despite its crucial importance in many biological, technological, and …

The present paper provides a theoretical analysis of the sum frequency generation (SFG)
spectrum of the water surface in the OH stretch mode frequency region based on ab initio …

This paper reviews aspects of nonlinear optical spectroscopy of interfaces. The emphasis is
put on second-order nonlinear optical techniques, such as sum-frequency generation (SFG) …

During the past decade vibrational sum frequency generation as a method to study
interfaces has matured and can now be applied more routinely to systems of increasing …

The advent of laser-based sources of ultrafast infrared pulses has extended the study of very
fast molecular dynamics to the observation of processes manifested through their effects on …

The chemistry that occurs at surfaces has been an intense area of study for many years
owing to its complexity and importance in describing a wide range of physical phenomena …

An important issue for developing a molecular-level mechanism of heterogeneous
interactions at the aqueous interface is determining changes in the interface with changes in …