Quantum-coherent nanoscience

AJ Heinrich, WD Oliver, LMK Vandersypen… - Nature …, 2021 - nature.com
For the past three decades nanoscience has widely affected many areas in physics,
chemistry and engineering, and has led to numerous fundamental discoveries, as well as …

Single-molecule magnets beyond a single lanthanide ion: the art of coupling

YC Chen, ML Tong - Chemical Science, 2022 - pubs.rsc.org
The promising future of storing and processing quantized information at the molecular level
has been attracting the study of Single-Molecule Magnets (SMMs) for almost three decades …

Computational design of magnetic molecules and their environment using quantum chemistry, machine learning and multiscale simulations

A Lunghi, S Sanvito - Nature Reviews Chemistry, 2022 - nature.com
Having served as a playground for fundamental studies on the physics of d and f electrons
for almost a century, magnetic molecules are now becoming increasingly important for …

Toward exact predictions of spin-phonon relaxation times: An ab initio implementation of open quantum systems theory

A Lunghi - Science Advances, 2022 - science.org
Spin-phonon coupling is the main driver of spin relaxation and decoherence in solid-state
semiconductors at finite temperature. Controlling this interaction is a central problem for …

Proof-of-Concept Quantum Simulator Based on Molecular Spin Qudits

S Chicco, G Allodi, A Chiesa, E Garlatti… - Journal of the …, 2023 - ACS Publications
The use of d-level qudits instead of two-level qubits can largely increase the power of
quantum logic for many applications, ranging from quantum simulations to quantum error …

Modular approach to creating functionalized surface arrays of molecular qubits

L Tesi, F Stemmler, M Winkler, SSY Liu… - Advanced …, 2023 - Wiley Online Library
The quest for developing quantum technologies is driven by the promise of exponentially
faster computations, ultrahigh performance sensing, and achieving thorough understanding …

[HTML][HTML] Electronic structure and magnetic anisotropy design of functional metal complexes

A Raza, M Perfetti - Coordination Chemistry Reviews, 2023 - Elsevier
Chemical guidelines to target a well-defined electronic structure and magnetic anisotropy
are of primary importance in physics, chemistry and biology. Our literature overview …

A conjugated Schiff-base macrocycle weakens the transverse crystal field of air-stable dysprosium single-molecule magnets

S Liu, Y Gil, C Zhao, J Wu, Z Zhu, XL Li… - Inorganic Chemistry …, 2022 - pubs.rsc.org
Self-condensation of bifunctional 8-aminoquinoline-2-carbaldehyde templated by
dysprosium (III) ions followed by the replacement of axial ligands with triphenylsilanol in the …

Toward molecular spin qubit devices: Integration of magnetic molecules into solid-state devices

AA Fursina, A Sinitskii - ACS Applied Electronic Materials, 2023 - ACS Publications
We review the progress made in integrating magnetic molecules containing transition metal
ions into nanoelectronic solid-state devices and using them as molecular spin qubits …

Functional lanthanide complexes with N, N′-bis (2-hydroxybenzyl)-N, N′-bis (pyridin-2-ylmethyl) ethylenediamine (H2bbpen) derivatives: Coordination chemistry …

YX Qu, PY Liao, YC Chen, ML Tong - Coordination Chemistry Reviews, 2023 - Elsevier
Lanthanide complexes are among the most active frontiers of functional coordination
chemistry, especially due to their fascinating magnetic and optical properties. Among them …