MoS2 intrinsically show Pt-like hydrogen evolution reaction (HER) performance. Pristine
MoS2 displayed low HER activity, which was caused by low quantities of catalytic sites and …

Microkinetic modeling of heterogeneous catalysis serves as an efficient tool bridging atom-
scale first-principles calculations and macroscale industrial reactor simulations …

We report the operando imaging of the methyl radical mole fraction above a working
catalyst. Using photofragmentation laser-induced fluorescence (PF-LIF), we imaged methyl …

The advent of machine learning potentials (MLPs) provides a unique opportunity to access
simulation time scales and to directly compute physicochemical properties that are typically …

The methyl radical plays a central role in plasma-assisted hydrocarbon chemistry but is
challenging to detect due to its high reactivity and strongly pre-dissociative electronically …

The role of a solid surface for initiating gas-phase reactions is still not well understood. The
hydrogen atom (H) is an important intermediate in gas-phase ethane dehydrogenation and …

Many important chemically reacting systems are inherently multi-dimensional with spatial
and temporal variations in the thermochemical state, which can be strongly coupled to …

We combine near-surface molecular beam mass spectrometry—a probe of the gas phase
within hundreds of micrometers of catalyst surfaces—and surface-sensitive infrared …

This study investigates the NO reduction by H 2 on a Pd/Al 2 O 3 catalyst in a temperature
range of 100–300° C and NO/H 2 ratios from 0.5–2, aiming to gain a deeper understanding …

The chemical reaction network of low-temperature plasma-assisted oxidation of methane
(CH4) and ethylene (C2H4) with nickel oxide (NiO) was investigated in a heated plasma …