Plutonium oxide melt structure and covalency

SK Wilke, CJ Benmore, OLG Alderman, G Sivaraman… - Nature Materials, 2024 - nature.com
Advances in nuclear power reactors include the use of mixed oxide fuel, containing uranium
and plutonium oxides. The high-temperature behaviour and structure of PuO2–x above …

Insight into the Cationic Charge Distribution in U1–yzPuyAmzOx Mixed Oxides

P Fouquet-Métivier, L Medyk, F Lebreton… - Inorganic …, 2024 - ACS Publications
Uranium–plutonium mixed oxides, containing few mol% of Am, are currently studied as fuel
for Sodium Fast Reactors. The study of the O/M ratio of these fuels is of main interest, as its …

Multi-scale structural investigation of uranium-plutonium mixed oxides (U1-yPuy) O2-x with high plutonium content

MM Desagulier, J Martinez, PM Martin… - Journal of Nuclear …, 2023 - Elsevier
Uranium-Plutonium mixed oxides U 1-y Pu y O 2-x are considered as the reference fuels for
Sodium-cooled Fast neutron Reactors (SFRs). Nevertheless, there is a lack of experimental …

Quantitative phase-field simulation of Pu oxidation at low temperatures through a pragmatic strategy for coupling with thermodynamic and diffusion descriptions of …

S Ma, P Liu, L Zhang - Journal of Nuclear Materials, 2025 - Elsevier
In this letter, we developed a pragmatic strategy for coupling the phase-field model with the
thermodynamic/kinetic descriptions and applied it to quantitatively describe the complex …

Description of new correlations and databases for fuel performance codes to be applied to Am bearing fuels

P Van Uffelen, A Schubert, M Lainet, A Magni… - 2024 - re.public.polimi.it
In this deliverable, we outline the correlations and data that have been transferred to models
suitable for fuel performance codes (TRANSURANUS, GERMINAL) for the simulation of Am …

[HTML][HTML] Melting behaviour of mixed plutonium and iron oxides: An experimental study

L Casini, L Luzzi, A Lacima-Nadolnik, D Robba… - Nuclear Materials and …, 2024 - Elsevier
The present work describes original experimental results obtained on the melting and
solidification behaviour of mixed PuO 2–Fe 3 O 4 samples. The samples were laser-heated …

Liquidus curve of uranium–plutonium mixed oxide (MOX) system

L Burakovsky, DL Preston, AA Green - Frontiers in Nuclear …, 2025 - frontiersin.org
Mixed oxides of uranium and plutonium (MOX) are currently considered reference fuels for
the new generation of fast breeder reactors such as ASTRID. The key factor determining the …

Ambient melting behavior of stoichiometric uranium oxides

L Burakovsky, SD Ramsey, RS Baty - Frontiers in Nuclear …, 2024 - frontiersin.org
As UO2 is easily oxidized during the nuclear fuel cycle it is important to have a detailed
understanding of the structures and properties of the oxidation products. Experimental work …

First principle study of the physical properties of actinide oxides. A review

AY Galashev - Electrochemical Materials and Technologies. 2024. Vol …, 2024 - elar.urfu.ru
Reprocessing spent nuclear fuel creates the conditions for converting nuclear energy to a
clean and sustainable energy. Thermal conductors in reactors are molten salts, the safe use …

Systematic study of the structural, energetic and elastic properties of U1-yAmyO2-xcompounds using empirical interatomic potentials

BM Labonne, C Gueneau, M Bertolus - Physical Chemistry Chemical …, 2024 - pubs.rsc.org
Uranium-americium mixed oxides are envisaged as fuels or blankets for the transmutation of
americium in fast neutron reactors, which requires an accurate knowledge of their …