Progress and prospects in nonlinear extreme-ultraviolet and X-ray optics and spectroscopy

M Chergui, M Beye, S Mukamel, C Svetina… - Nature Reviews …, 2023 - nature.com
Free-electron lasers and high-harmonic-generation table-top systems are new sources of
extreme-ultraviolet to hard X-ray photons, providing ultrashort pulses that are intense …

Short-wavelength free-electron laser sources and science: a review

EA Seddon, JA Clarke, DJ Dunning… - Reports on Progress …, 2017 - iopscience.iop.org
This review is focused on free-electron lasers (FELs) in the hard to soft x-ray regime. The
aim is to provide newcomers to the area with insights into: the basic physics of FELs, the …

Roadmap of ultrafast x-ray atomic and molecular physics

L Young, K Ueda, M Gühr… - Journal of Physics B …, 2018 - iopscience.iop.org
X-ray free-electron lasers (XFELs) and table-top sources of x-rays based upon high
harmonic generation (HHG) have revolutionized the field of ultrafast x-ray atomic and …

High efficiency ultrafast water-window harmonic generation for single-shot soft X-ray spectroscopy

Y Fu, K Nishimura, R Shao, A Suda… - Communications …, 2020 - nature.com
Fully coherent, soft X-ray attosecond pulses are now available through high-order harmonic
generation (HHG); however, the output energy is insufficient for various applications, such …

Electronic population transfer via impulsive stimulated x-ray Raman scattering with attosecond soft-x-ray pulses

JT O'Neal, EG Champenois, S Oberli, R Obaid… - Physical review …, 2020 - APS
Free-electron lasers provide a source of x-ray pulses short enough and intense enough to
drive nonlinearities in molecular systems. Impulsive interactions driven by these x-ray pulses …

Non-linear processes in the extreme ultraviolet

I Orfanos, I Makos, I Liontos, E Skantzakis… - Journal of Physics …, 2020 - iopscience.iop.org
Recent developments in extreme ultraviolet (XUV) and x-ray radiation sources have pushed
pulse energies and durations to unprecedented levels that opened up the era of non-linear …

Application of a molecular networking approach for clinical and forensic toxicology exemplified in three cases involving 3‐MeO‐PCP, doxylamine, and chlormequat

S Allard, PM Allard, I Morel… - Drug testing and …, 2019 - Wiley Online Library
Untargeted toxicological screening is an analytical challenge, given the high number of
molecules and metabolites to be detected and the constant appearance of new …

Cherry-picking resolvents: Recovering the valence contribution in X-ray two-photon absorption within the core–valence-separated equation-of-motion coupled-cluster …

JH Andersen, KD Nanda, AI Krylov… - Journal of Chemical …, 2022 - ACS Publications
Calculations of first-order response wave functions in the X-ray regime often diverge within
correlated frameworks such as equation-of-motion coupled-cluster singles and doubles …

Nonlinear spectroscopy with X-ray two-photon absorption in metallic copper

K Tamasaku, E Shigemasa, Y Inubushi, I Inoue… - Physical Review Letters, 2018 - APS
X-ray two-photon absorption (TPA) spectrum of metallic copper is measured using a free-
electron laser (XFEL). The spectrum differs from that measured by the conventional one …

Shortening x-ray pulse duration via saturable absorption

I Inoue, Y Inubushi, T Osaka, J Yamada, K Tamasaku… - Physical Review Letters, 2021 - APS
To shorten the duration of x-ray pulses, we present a nonlinear optical technique using
atoms with core-hole vacancies (core-hole atoms) generated by inner-shell photoionization …