Ultrafast electron diffraction: Visualizing dynamic states of matter

D Filippetto, P Musumeci, RK Li, BJ Siwick… - Reviews of Modern …, 2022 - APS
Since the discovery of electron-wave duality, electron scattering instrumentation has
developed into a powerful array of techniques for revealing the atomic structure of matter …

Femtosecond electron diffraction: heralding the era of atomically resolved dynamics

G Sciaini, RJD Miller - Reports on Progress in Physics, 2011 - iopscience.iop.org
One of the great dream experiments in Science is to directly observe atomic motions as they
occur. Femtosecond electron diffraction provided the first'light'of sufficient intensity to …

Attosecond electron microscopy and diffraction

D Hui, H Alqattan, M Sennary, NV Golubev… - Science …, 2024 - science.org
Advances in attosecond spectroscopy have enabled tracing and controlling the electron
motion dynamics in matter, although they have yielded insufficient information about the …

Femtosecond crystallography with ultrabright electrons and x-rays: Capturing chemistry in action

RJD Miller - Science, 2014 - science.org
With the recent advances in ultrabright electron and x-ray sources, it is now possible to
extend crystallography to the femtosecond time domain to literally light up atomic motions …

An atomic-level view of melting using femtosecond electron diffraction

BJ Siwick, JR Dwyer, RE Jordan, RJD Miller - Science, 2003 - science.org
We used 600-femtosecond electron pulses to study the structural evolution of aluminum as it
underwent an ultrafast laser–induced solid-liquid phase transition. Real-time observations …

Photon-induced near-field electron microscopy (PINEM): theoretical and experimental

ST Park, M Lin, AH Zewail - New Journal of Physics, 2010 - iopscience.iop.org
Electron imaging in space and time is achieved in microscopy with timed (near relativistic)
electron packets of picometer wavelength coincident with light pulses of femtosecond …

Coulomb-correlated electron number states in a transmission electron microscope beam

R Haindl, A Feist, T Domröse, M Möller, JH Gaida… - Nature Physics, 2023 - nature.com
While correlated electrons are at the heart of many phenomena in condensed matter, as well
as atomic and molecular physics, Coulomb interactions in free-electron beams are generally …

Ultrafast electron microscopy in materials science, biology, and chemistry

WE King, GH Campbell, A Frank, B Reed… - Journal of Applied …, 2005 - pubs.aip.org
The use of pump-probe experiments to study complex transient events has been an area of
significant interest in materials science, biology, and chemistry. While the emphasis has …

Capturing chemistry in action with electrons: realization of atomically resolved reaction dynamics

AA Ischenko, PM Weber, RJD Miller - Chemical reviews, 2017 - ACS Publications
One of the grand challenges in chemistry has been to directly observe atomic motions
during chemical processes. The depiction of the nuclear configurations in space-time to …

Electron source concept for single-shot sub-100 fs electron diffraction in the 100 keV range

T Van Oudheusden, EF De Jong… - Journal of Applied …, 2007 - pubs.aip.org
We present a method for producing sub-100 fs electron bunches that are suitable for single-
shot ultrafast electron diffraction experiments in the 100 keV energy range. A combination of …