Ultrafast electron diffraction: Visualizing dynamic states of matter

D Filippetto, P Musumeci, RK Li, BJ Siwick… - Reviews of Modern …, 2022 - APS
Since the discovery of electron-wave duality, electron scattering instrumentation has
developed into a powerful array of techniques for revealing the atomic structure of matter …

4D ultrafast electron diffraction, crystallography, and microscopy

AH Zewail - Annu. Rev. Phys. Chem., 2006 - annualreviews.org
▪ Abstract In this review, we highlight the progress made in the development of 4D ultrafast
electron diffraction (UED), crystallography (UEC), and microscopy (UEM) with a focus on …

An atomic-level view of melting using femtosecond electron diffraction

BJ Siwick, JR Dwyer, RE Jordan, RJD Miller - Science, 2003 - science.org
We used 600-femtosecond electron pulses to study the structural evolution of aluminum as it
underwent an ultrafast laser–induced solid-liquid phase transition. Real-time observations …

Ultrafast electron microscopy in materials science, biology, and chemistry

WE King, GH Campbell, A Frank, B Reed… - Journal of Applied …, 2005 - pubs.aip.org
The use of pump-probe experiments to study complex transient events has been an area of
significant interest in materials science, biology, and chemistry. While the emphasis has …

Capturing chemistry in action with electrons: realization of atomically resolved reaction dynamics

AA Ischenko, PM Weber, RJD Miller - Chemical reviews, 2017 - ACS Publications
One of the grand challenges in chemistry has been to directly observe atomic motions
during chemical processes. The depiction of the nuclear configurations in space-time to …

Ultrafast time-resolved electron diffraction with megavolt electron beams

JB Hastings, FM Rudakov, DH Dowell… - Applied physics …, 2006 - pubs.aip.org
A rf photocathode electron gun is used as an electron source for ultrafast time-resolved
pump-probe electron diffraction. The authors observed single-shot diffraction patterns from a …

Ultrafast electron crystallography of interfacial water

CY Ruan, VA Lobastov, F Vigliotti, S Chen, AH Zewail - Science, 2004 - science.org
We report direct determination of the structures and dynamics of interfacial water on a
hydrophilic surface with atomic-scale resolution using ultrafast electron crystallography. On …

Femtosecond electron diffraction:'making the molecular movie'

JR Dwyer, CT Hebeisen… - … of the Royal …, 2006 - royalsocietypublishing.org
Femtosecond electron diffraction (FED) has the potential to directly observe transition state
processes. The relevant motions for this barrier-crossing event occur on the hundred …

Breaking resolution limits in ultrafast electron diffraction and microscopy

P Baum, AH Zewail - … of the National Academy of Sciences, 2006 - National Acad Sciences
Ultrafast electron microscopy and diffraction are powerful techniques for the study of the time-
resolved structures of molecules, materials, and biological systems. Central to these …

Attosecond electron pulses for 4D diffraction and microscopy

P Baum, AH Zewail - … of the National Academy of Sciences, 2007 - National Acad Sciences
In this contribution, we consider the advancement of ultrafast electron diffraction and
microscopy to cover the attosecond time domain. The concept is centered on the …