Fracture and adhesion of soft materials: a review

C Creton, M Ciccotti - Reports on Progress in Physics, 2016 - iopscience.iop.org
Soft materials are materials with a low shear modulus relative to their bulk modulus and
where elastic restoring forces are mainly of entropic origin. A sparse population of strong …

Bioinspired polymer systems with stimuli-responsive mechanical properties

L Montero de Espinosa, W Meesorn, D Moatsou… - Chemical …, 2017 - ACS Publications
Materials with switchable mechanical properties are widespread in living organisms and
endow many species with traits that are essential for their survival. Many of the mechanically …

50th anniversary perspective: Networks and gels: Soft but dynamic and tough

C Creton - Macromolecules, 2017 - ACS Publications
Soft polymer networks have seen an explosion of recent developments motivated by new
high tech applications in the biomedical field or in engineering. We present a candid and …

Multi-scale multi-mechanism design of tough hydrogels: building dissipation into stretchy networks

X Zhao - Soft matter, 2014 - pubs.rsc.org
As swollen polymer networks in water, hydrogels are usually brittle. However, hydrogels with
high toughness play critical roles in many plant and animal tissues as well as in diverse …

High-strength, tough, fatigue resistant, and self-healing hydrogel based on dual physically cross-linked network

Z Gong, G Zhang, X Zeng, J Li, G Li… - … applied materials & …, 2016 - ACS Publications
Hydrogels usually suffer from low mechanical strength, which largely limit their application in
many fields. In this Research Article, we prepared a dual physically cross-linked hydrogel …

Self-healable, tough, and ultrastretchable nanocomposite hydrogels based on reversible polyacrylamide/montmorillonite adsorption

G Gao, G Du, Y Sun, J Fu - ACS applied materials & interfaces, 2015 - ACS Publications
Nanocomposite hydrogels with unprecedented stretchability, toughness, and self-healing
have been developed by in situ polymerization of acrylamide with the presence of exfoliated …

Mineral-enhanced polyacrylic acid hydrogel as an oyster-inspired organic–inorganic hybrid adhesive

A Li, Y Jia, S Sun, Y Xu, BB Minsky… - … applied materials & …, 2018 - ACS Publications
Underwater adhesion is crucial to many marine life forms living a sedentary lifestyle.
Amongst them, mussel adhesion has been mostly studied, which inspires numerous …

Hydrophilicity‐hydrophobicity transformation, thermoresponsive morphomechanics, and crack multifurcation revealed by AIEgens in mechanically strong hydrogels

Y Hu, L Barbier, Z Li, X Ji, H Le Blay… - Advanced …, 2021 - Wiley Online Library
Biomimetic exploration of stimuli‐responsive and crack‐resistant hydrogels is of great
academic and practical significance, although the rational design of tough hydrogels is …

Modern strategies to achieve tissue-mimetic, mechanically robust hydrogels

AK Means, MA Grunlan - 2019 - ACS Publications
Hydrogels are frequently used biomaterials due to their similarity in hydration and structure
to biological tissues. However, their utility is limited by poor mechanical properties, namely …

Cellulose nanocrystals mechanical reinforcement in composite hydrogels with multiple cross-links: correlations between dissipation properties and deformation …

J Yang, CR Han, XM Zhang, F Xu, RC Sun - Macromolecules, 2014 - ACS Publications
Nanocomposites have drawn a great interest in materials science of elastomers in recent
years, and tailoring interfacial interactions between fillers and polymer matrix plays a critical …