Four-dimensional electron microscopy: Ultrafast imaging, diffraction and spectroscopy in materials science and biology

GM Vanacore, AWP Fitzpatrick, AH Zewail - Nano Today, 2016 - Elsevier
Understanding the ultrafast evolution of atomic and electronic rearrangements under
nonequilibrium conditions in organic, inorganic and biological materials plays a …

Electron-phonon coupling and energy flow in a simple metal beyond the two-temperature approximation

L Waldecker, R Bertoni, R Ernstorfer, J Vorberger - Physical Review X, 2016 - APS
The electron-phonon coupling and the corresponding energy exchange are investigated
experimentally and by ab initio theory in nonequilibrium states of the free-electron metal …

[HTML][HTML] Structural dynamics at surfaces by ultrafast reflection high-energy electron diffraction

M Horn-von Hoegen - Structural Dynamics, 2024 - pubs.aip.org
Many fundamental processes of structural changes at surfaces occur on a pico-or
femtosecond timescale. In order to study such ultrafast processes, we have combined …

[HTML][HTML] Nanoscale diffractive probing of strain dynamics in ultrafast transmission electron microscopy

A Feist, N Rubiano da Silva, W Liang, C Ropers… - Structural …, 2018 - pubs.aip.org
The control of optically driven high-frequency strain waves in nanostructured systems is an
essential ingredient for the further development of nanophononics. However, broadly …

Rippling ultrafast dynamics of suspended 2D monolayers, graphene

J Hu, GM Vanacore, A Cepellotti… - Proceedings of the …, 2016 - National Acad Sciences
Here, using ultrafast electron crystallography (UEC), we report the observation of rippling
dynamics in suspended monolayer graphene, the prototypical and most-studied 2D …

[HTML][HTML] Coulomb interactions in high-coherence femtosecond electron pulses from tip emitters

N Bach, T Domröse, A Feist, T Rittmann… - Structural …, 2019 - pubs.aip.org
Tip-based photoemission electron sources offer unique properties for ultrafast imaging,
diffraction, and spectroscopy experiments with highly coherent few-electron pulses …

Spatio-temporal resolution studies on a highly compact ultrafast electron diffractometer

C Gerbig, A Senftleben, S Morgenstern… - New Journal of …, 2015 - iopscience.iop.org
Time-resolved diffraction with femtosecond electron pulses has become a promising
technique to directly provide insights into photo induced primary dynamics at the atomic …

[HTML][HTML] Femtosecond single-electron diffraction

S Lahme, C Kealhofer, F Krausz, P Baum - Structural Dynamics, 2014 - pubs.aip.org
Ultrafast electron diffraction allows the tracking of atomic motion in real time, but space
charge effects within dense electron packets are a problem for temporal resolution. Here, we …

[HTML][HTML] Ultrafast core-loss spectroscopy in four-dimensional electron microscopy

RM van der Veen, TJ Penfold, AH Zewail - Structural dynamics, 2015 - pubs.aip.org
We demonstrate ultrafast core-electron energy-loss spectroscopy in four-dimensional
electron microscopy as an element-specific probe of nanoscale dynamics. We apply it to the …

An ultrafast electron microscope gun driven by two-photon photoemission from a nanotip cathode

R Bormann, S Strauch, S Schäfer… - Journal of Applied Physics, 2015 - pubs.aip.org
We experimentally and numerically investigate the performance of an advanced ultrafast
electron source, based on two-photon photoemission from a tungsten needle cathode …