Magnetic axiality: design principles from molecules to materials

KLM Harriman, D Errulat, M Murugesu - Trends in Chemistry, 2019 - cell.com
Recently, the field of molecular magnets has experienced a remarkable result: magnetic
remanence above liquid nitrogen temperatures (> 77 K); this represents the first example of …

Reading and writing single-atom magnets

FD Natterer, K Yang, W Paul, P Willke, T Choi, T Greber… - Nature, 2017 - nature.com
The single-atom bit represents the ultimate limit of the classical approach to high-density
magnetic storage media. So far, the smallest individually addressable bistable magnetic bits …

Spin decoherence of magnetic atoms on surfaces

F Delgado, J Fernández-Rossier - Progress in Surface Science, 2017 - Elsevier
We review the problem of spin decoherence of magnetic atoms deposited on a surface.
Recent breakthroughs in scanning tunnelling microscopy (STM) make it possible to probe …

Magnetic remanence in single atoms

F Donati, S Rusponi, S Stepanow, C Wäckerlin… - Science, 2016 - science.org
A permanent magnet retains a substantial fraction of its saturation magnetization in the
absence of an external magnetic field. Realizing magnetic remanence in a single atom …

Control of the millisecond spin lifetime of an electrically probed atom

W Paul, K Yang, S Baumann, N Romming, T Choi… - Nature Physics, 2017 - nature.com
Electrical control and readout of magnetic states is an important goal in spintronics. But
electrical access to quantum spin systems comes at the cost of coupling to electrodes, which …

Slow magnetic relaxation of Dy adatoms with in-plane magnetic anisotropy on a two-dimensional electron gas

V Bellini, S Rusponi, J Kolorenč, SK Mahatha… - ACS …, 2022 - ACS Publications
We report on the magnetic properties of Dy atoms adsorbed on the (001) surface of SrTiO3.
X-ray magnetic circular dichroism reveals slow relaxation of the Dy magnetization on a time …

Measuring the intra-atomic exchange energy in rare-earth adatoms

M Pivetta, F Patthey, I Di Marco, A Subramonian… - Physical Review X, 2020 - APS
We present the first experimental determination of the intra-atomic exchange energy
between the inner 4 f and the outer 6 s 5 d shells in rare-earth elements. Inelastic electron …

A perspective on surface-adsorbed single atom magnets as atomic-scale magnetic memory

F Donati, AJ Heinrich - Applied Physics Letters, 2021 - pubs.aip.org
Downscaling single magnetic bits to the ultimate size of individual atoms would open the
possibility to maximize the magnetic storage density on a solid surface. However, realizing …

occupancy and magnetism of rare-earth atoms adsorbed on metal substrates

A Singha, R Baltic, F Donati, C Wäckerlin, J Dreiser… - Physical Review B, 2017 - APS
We report x-ray absorption spectroscopy and x-ray magnetic circular dichroism
measurements as well as multiplet calculations for Dy, Ho, Er, and Tm atoms adsorbed on Pt …

An orbitally derived single-atom magnetic memory

B Kiraly, AN Rudenko, WMJ van Weerdenburg… - Nature …, 2018 - nature.com
A magnetic atom epitomizes the scaling limit for magnetic information storage. Individual
atomic spins have recently exhibited magnetic remanence, a requirement for magnetic …