Spontaneous exciton dissociation in transition metal dichalcogenide monolayers

T Handa, M Holbrook, N Olsen, LN Holtzman… - Science …, 2024 - science.org
Since the seminal work on MoS2, photoexcitation in atomically thin transition metal
dichalcogenides (TMDCs) has been assumed to result in excitons, with binding energies …

Control of the bright-dark exciton splitting using the Lamb shift in a two-dimensional semiconductor

L Ren, C Robert, M Glazov, M Semina, T Amand… - Physical Review Letters, 2023 - APS
We investigate the exciton fine structure in atomically thin WSe 2-based van der Waals
heterostructures where the density of optical modes at the location of the semiconductor …

Interaction-driven transport of dark excitons in 2D semiconductors with phonon-mediated optical readout

SB Chand, JM Woods, J Quan, E Mejia… - Nature …, 2023 - nature.com
The growing field of quantum information technology requires propagation of information
over long distances with efficient readout mechanisms. Excitonic quantum fluids have …

Strain control of exciton and trion spin-valley dynamics in monolayer transition metal dichalcogenides

Z An, P Soubelet, Y Zhumagulov, M Zopf, A Delhomme… - Physical Review B, 2023 - APS
The electron-hole exchange interaction is a fundamental mechanism that drives valley
depolarization via intervalley exciton hopping in semiconductor multivalley systems. Here …

Efficient electron spin relaxation by chiral phonons in monolayers

D Lagarde, M Glazov, V Jindal, K Mourzidis, I Gerber… - Physical Review B, 2024 - APS
In transition metal dichalcogenide semiconductor monolayers the spin dynamics of electrons
is controlled by the original spin-valley locking effect resulting from the interplay between …

Ab initio quantum approach to electron-hole exchange for semiconductors hosting Wannier excitons

M Combescot, T Amand, SY Shiau - Physical Review B, 2023 - APS
We propose a quantum approach to “electron-hole exchange,” better named electron-hole
pair exchange, that makes use of the second quantization formalism to describe the problem …

Essential role of momentum-forbidden dark excitons in the energy transfer responses of monolayer transition-metal dichalcogenides

JD Lin, PY Lo, GH Peng, WH Li, SY Huang… - npj 2D Materials and …, 2023 - nature.com
We present a theoretical investigation of exciton-mediated Förster resonant energy transfers
(FRET's) from photoexcited quantum dots (QD's) to transition-metal dichalcogenide …

Perspective on trions and excitons in two-dimensional atomically thin materials

YV Zhumagulov, V Perebeinos - Applied Physics Letters, 2024 - pubs.aip.org
Charged excitons or trions are essential for optical spectra in low-dimensional doped
monolayers of transitional metal dichalcogenides. This Perspective aims to provide an …

Observation of Multi-Phonon Emission in Monolayer WS2 on Various Substrates

ER Adler, TDM Le, I Boulares, R Boyd, Y He, D Rhodes… - Nanomaterials, 2023 - mdpi.com
Transition metal dichalcogenides (TMDs) have unique absorption and emission properties
that stem from their large excitonic binding energies, reduced-dielectric screening, and …

Energy shifts and broadening of excitonic resonances in electrostatically-doped semiconductors

H Dery, C Robert, SA Crooker, X Marie… - arXiv preprint arXiv …, 2024 - arxiv.org
Tuning the density of resident electrons or holes in semiconductors provides crucial insight
into the composition of excitonic complexes that are observed as absorption or …