Getting the Most Out of Fluorogenic Probes: Challenges and Opportunities in Using Single-Molecule Fluorescence to Image Electro-and Photocatalysis

M Shen, WH Rackers, B Sadtler - Chemical & Biomedical Imaging, 2023 - ACS Publications
Single-molecule fluorescence microscopy enables the direct observation of individual
reaction events at the surface of a catalyst. It has become a powerful tool to image in real …

Elucidating the weakly reversible Cs–Pb–Br perovskite nanocrystal reaction network with high-throughput maps and transformations

JC Dahl, X Wang, X Huang, EM Chan… - Journal of the …, 2020 - ACS Publications
Advances in automation and data analytics can aid exploration of the complex chemistry of
nanoparticles. Lead halide perovskite colloidal nanocrystals provide an interesting proving …

Precursor chemistry of lead bromide perovskite nanocrystals

JC Dahl, EB Curling, M Loipersberger, JJ Calvin… - ACS …, 2024 - ACS Publications
We investigate the early stages of cesium lead bromide perovskite formation through
absorption spectroscopy of stopped-flow reactions, high-throughput mapping, and direct …

Single‐Photon Emission from Single Microplate MAPbI3 Nanocrystals with Ultranarrow Photoluminescence Linewidths and Exciton Fine Structures

J Yuan, D Zhou, C Zhuang, Y Zhou… - Advanced Optical …, 2022 - Wiley Online Library
Stimulated by the superior performance of organic–inorganic MAPbI3 perovskite films in
photovoltaic devices, a lot of research interest is now being devoted to their low …

Role of solid-state miscibility during anion exchange in cesium lead halide nanocrystals probed by single-particle fluorescence

D Wang, J Cavin, B Yin, AS Thind… - The journal of …, 2020 - ACS Publications
In this Letter, we used fluorescence microscopy to image the reversible transformation of
individual CsPbCl3 nanocrystals to CsPbBr3, which enables us to quantify heterogeneity in …

Size-dependent miscibility controls the kinetics of anion exchange in cesium lead halide nanocrystals

D Zhang, XS Wu, D Wang, B Sadtler - The Journal of Chemical Physics, 2023 - pubs.aip.org
Anion exchange is a facile, post-synthetic method to tune the emission wavelength of
colloidal cesium lead halide (CsPbX 3, X= Cl, Br, I) perovskite nanocrystals. While colloidal …

Stochastic noise in single-nanoparticle catalysis

D Devasia, PK Jain - The Journal of Physical Chemistry C, 2021 - ACS Publications
Nanoparticle-based catalysts exhibit considerable complexity and heterogeneity. New light
can be shed into these aspects by probing catalysis on the level of single nanoparticles …

Irreversibility in anion exchange between cesium lead bromide and iodide nanocrystals imaged by single-particle fluorescence

D Wang, D Zhang, B Sadtler - The Journal of Physical Chemistry …, 2020 - ACS Publications
Anion exchange is a powerful method to tune the emission wavelength of perovskite
CsPbX3 (X= Cl, Br, or I) nanocrystals across the visible spectrum. CsPbX3 nanocrystals can …

Label-free tracking of photocatalysis on a single nanoparticle

D Devasia - 2021 - ideals.illinois.edu
Nanocatalysis is a rapidly growing field where nanoparticles are exploited to catalyze
industrially relevant chemical reactions. The successful design of these heterogeneous …

[图书][B] Formation and Transformation of Colloidal Metal Halide Nanoparticles

JC Dahl - 2022 - search.proquest.com
Colloidal nanocrystals are miniscule pieces (< 100 nm or∼ 1/1000th the width of a human
hair) of solid materials suspended in a liquid. Semiconductor nanocrystals have controllable …