Quantum Many-Body Theory from a Solution of the -Representability Problem

DA Mazziotti - Physical Review Letters, 2023 - APS
Here we present a many-body theory based on a solution of the N-representability problem
in which the ground-state two-particle reduced density matrix (2-RDM) is determined directly …

A Molecular Perspective of Exciton Condensation from Particle-Hole Reduced Density Matrices

LI Payne Torres, AO Schouten… - The Journal of …, 2024 - ACS Publications
Exciton condensation, the Bose–Einstein-like condensation of quasibosonic particle-hole
pairs, has been the subject of much theoretical and experimental interest and holds promise …

Exciton-condensate-like amplification of energy transport in light harvesting

AO Schouten, LAM Sager-Smith, DA Mazziotti - PRX Energy, 2023 - APS
Bose-Einstein condensation of excitons, in which excitons condense into a single coherent
quantum state, known as an exciton condensate, enables frictionless energy transfer, but …

Molecular origins of exciton condensation in van der Waals heterostructure bilayers

LIP Torres, AO Schouten, DA Mazziotti - Chemical Science, 2024 - pubs.rsc.org
Recent experiments have realized exciton condensation in bilayer materials such as
graphene double layers and the van der Waals heterostructure MoSe2–WSe2 with the …

Potential for exciton condensation in a highly conductive amorphous polymer

AO Schouten, JE Klevens, LAM Sager-Smith, J Xie… - Physical Review …, 2023 - APS
An outstanding challenge in synthesis and theory is to develop molecular materials at
ambient conditions that exhibit highly efficient energy transfer. Here we demonstrate the …

Large cumulant eigenvalue as a signature of exciton condensation

AO Schouten, LAM Sager-Smith, DA Mazziotti - Physical Review B, 2022 - APS
The Bose-Einstein condensation of excitons into a single quantum state is known as exciton
condensation. Exciton condensation, which potentially supports the frictionless flow of …

Quantum phase transitions in a model Hamiltonian exhibiting entangled simultaneous fermion-pair and exciton condensations

S Warren, LAM Sager-Smith, DA Mazziotti - Physical Review B, 2022 - APS
Quantum states of a novel Bose-Einstein condensate, in which both fermion-pair and exciton
condensations are simultaneously present, have recently been realized theoretically in a …

A Pair of 2D Quantum Liquids: Investigating the Phase Behavior of Indirect Excitons

PR Wrona, E Rabani, PL Geissler - ACS nano, 2022 - ACS Publications
Long-lived indirect excitons (IXs) exhibit a rich phase diagram, including a Bose–Einstein
condensate (BEC), a Wigner crystal, and other exotic phases. Recent experiments have …

Exploration of Highly-Correlated Systems on Classical and Quantum Devices

LAM Sager-Smith - 2023 - search.proquest.com
Elucidation of many chemical behaviors and properties depends on our ability to model the
physics of electron-electron interactions at reasonable computational expense with …