New frontiers for quantum gases of polar molecules

SA Moses, JP Covey, MT Miecnikowski, DS Jin, J Ye - Nature Physics, 2017 - nature.com
Compared to atoms, molecules possess additional degrees of freedom that can be exploited
in fundamental tests, ultracold chemistry, and engineering new quantum phases in many …

Robust storage qubits in ultracold polar molecules

PD Gregory, JA Blackmore, SL Bromley, JM Hutson… - Nature Physics, 2021 - nature.com
Quantum states with long-lived coherence are essential for quantum computation,
simulation and metrology. The nuclear spin states of ultracold molecules prepared in the …

Second-scale rotational coherence and dipolar interactions in a gas of ultracold polar molecules

PD Gregory, LM Fernley, AL Tao, SL Bromley, J Stepp… - Nature Physics, 2024 - nature.com
Ultracold polar molecules combine a rich structure of long-lived internal states with access to
controllable long-range anisotropic dipole–dipole interactions. In particular, the rotational …

Ultracold molecules for quantum simulation: rotational coherences in CaF and RbCs

JA Blackmore, L Caldwell, PD Gregory… - Quantum Science …, 2018 - iopscience.iop.org
Polar molecules offer a new platform for quantum simulation of systems with long-range
interactions, based on the electrostatic interaction between their electric dipole moments …

Observation of Rydberg blockade due to the charge-dipole interaction between an atom and a polar molecule

A Guttridge, DK Ruttley, AC Baldock… - Physical Review Letters, 2023 - APS
We demonstrate Rydberg blockade due to the charge-dipole interaction between a single
Rb atom and a single RbCs molecule confined in optical tweezers. The molecule is formed …

Loss of Ultracold Molecules via Optical Excitation of Long-Lived Two-Body Collision Complexes

PD Gregory, JA Blackmore, SL Bromley, SL Cornish - Physical Review Letters, 2020 - APS
We show that the lifetime of ultracold ground-state Rb 87 Cs 133 molecules in an optical trap
is limited by fast optical excitation of long-lived two-body collision complexes. We partially …

Enhanced quantum control of individual ultracold molecules using optical tweezer arrays

DK Ruttley, A Guttridge, TR Hepworth, SL Cornish - PRX Quantum, 2024 - APS
Control over the quantum states of individual molecules is crucial in the quest to harness
their rich internal structure and dipolar interactions for applications in quantum science. In …

Molecule–molecule and atom–molecule collisions with ultracold RbCs molecules

PD Gregory, JA Blackmore, LM Fernley… - New Journal of …, 2021 - iopscience.iop.org
Understanding ultracold collisions involving molecules is of fundamental importance for
current experiments, where inelastic collisions typically limit the lifetime of molecular …

Efficient conversion of closed-channel-dominated Feshbach molecules of to their absolute ground state

R Bause, A Kamijo, XY Chen, M Duda, A Schindewolf… - Physical Review A, 2021 - APS
We demonstrate the transfer of Na 23 K 40 molecules from a closed-channel-dominated
Feshbach-molecule state to the absolute ground state. The Feshbach molecules are initially …

Controlling the rotational and hyperfine state of ultracold molecules

PD Gregory, J Aldegunde, JM Hutson, SL Cornish - Physical Review A, 2016 - APS
We demonstrate coherent control of the rotational and hyperfine state of ultracold,
chemically stable Rb 87 Cs 133 molecules with external microwave fields. We create a …