Quantum control of molecular rotation

CP Koch, M Lemeshko, D Sugny - Reviews of Modern Physics, 2019 - APS
The angular momentum of molecules, or, equivalently, their rotation in three-dimensional
space, is ideally suited for quantum control. Molecular angular momentum is naturally …

Training Schrödinger's cat: Quantum optimal control: Strategic report on current status, visions and goals for research in Europe

SJ Glaser, U Boscain, T Calarco, CP Koch… - The European Physical …, 2015 - Springer
It is control that turns scientific knowledge into useful technology: in physics and engineering
it provides a systematic way for driving a dynamical system from a given initial state into a …

Quantum control of field-free molecular orientation

QQ Hong, ZZ Lian, CC Shu… - Physical Chemistry …, 2023 - pubs.rsc.org
Generating field-free (non-stationary) orientation of molecules in space has been a
longstanding goal in the field of quantum control of molecular rotation, which has significant …

High degree of molecular orientation by a combination of THz and femtosecond laser pulses

K Kitano, N Ishii, J Itatani - Physical Review A—Atomic, Molecular, and Optical …, 2011 - APS
We propose a method for achieving molecular orientation by two-step excitation with intense
femtosecond laser and terahertz (THz) pulses. First, the femtosecond laser pulse induces off …

Dynamics of molecules in extreme rotational states

L Yuan, SW Teitelbaum… - Proceedings of the …, 2011 - National Acad Sciences
We have constructed an optical centrifuge with a pulse energy that is more than 2 orders of
magnitude larger than previously reported instruments. This high pulse energy enables us to …

Orientational quantum revivals induced by a single-cycle terahertz pulse

CC Shu, QQ Hong, Y Guo, NE Henriksen - Physical Review A, 2020 - APS
The phenomenon of quantum revivals resulting from the self-interference of wave packets
has been observed in several quantum systems and utilized widely in spectroscopic …

Generation of maximal three-state field-free molecular orientation with terahertz pulses

QQ Hong, LB Fan, CC Shu, NE Henriksen - Physical Review A, 2021 - APS
We present a combined analytical and numerical investigation to show how an optimal
control field can be designed to generate maximum field-free orientation of molecules for …

Selective Ionization of Oriented Nonpolar Molecules with Asymmetric Structure<? format?> by Phase-Controlled Two-Color Laser Fields

H Ohmura, N Saito, M Tachiya - Physical review letters, 2006 - APS
We report on the selective ionization of oriented nonpolar molecules with asymmetric
structure by using phase-controlled two-color ω+ 2 ω laser pulses with an intensity of 1.0× …

Field-free molecular orientation induced by single-cycle THz pulses: The role of resonance and quantum interference

CC Shu, NE Henriksen - Physical Review A—Atomic, Molecular, and Optical …, 2013 - APS
We consider the rotational excitation of molecules induced by asymmetric (“half-cycle”) as
well as symmetric single-cycle THz pulses, leading to field-free time-dependent orientation …

Monotonic parareal control for quantum systems

Y Maday, J Salomon, G Turinici - SIAM Journal on Numerical Analysis, 2007 - SIAM
Following encouraging experimental results in quantum control, numerical simulations have
known significant improvements through the introduction of efficient optimization algorithms …