Promises and challenges of next-generation “beyond Li-ion” batteries for electric vehicles and grid decarbonization

Y Tian, G Zeng, A Rutt, T Shi, H Kim, J Wang… - Chemical …, 2020 - ACS Publications
The tremendous improvement in performance and cost of lithium-ion batteries (LIBs) have
made them the technology of choice for electrical energy storage. While established battery …

Physicochemical concepts of the lithium metal anode in solid-state batteries

T Krauskopf, FH Richter, WG Zeier, J Janek - Chemical reviews, 2020 - ACS Publications
Developing reversible lithium metal anodes with high rate capability is one of the central
aims of current battery research. Lithium metal anodes are not only required for the …

Electrochemical impedance spectroscopy for all‐solid‐state batteries: Theory, methods and future outlook

P Vadhva, J Hu, MJ Johnson, R Stocker… - …, 2021 - Wiley Online Library
Electrochemical impedance spectroscopy (EIS) is widely used to probe the physical and
chemical processes in lithium (Li)‐ion batteries (LiBs). The key parameters include state‐of …

Innovative approaches to Li-argyrodite solid electrolytes for all-solid-state lithium batteries

L Zhou, N Minafra, WG Zeier… - Accounts of Chemical …, 2021 - ACS Publications
Conspectus As the world transitions away from fossil energy to green and renewable
energy, electrochemical energy storage increasingly becomes a vital component of the mix …

Challenges of today for Na-based batteries of the future: From materials to cell metrics

I Hasa, S Mariyappan, D Saurel, P Adelhelm… - Journal of Power …, 2021 - Elsevier
Several emerging battery technologies are currently on endeavour to take a share of the
dominant position taken by Li-ion batteries in the field of energy storage. Among them …

Electrochemical ion insertion from the atomic to the device scale

A Sood, AD Poletayev, DA Cogswell… - Nature Reviews …, 2021 - nature.com
Electrochemical ion insertion involves coupled ion–electron transfer reactions, transport of
guest species and redox of the host. The hosts are typically anisotropic solids with 2D …

Energy storage materials for solid‐state batteries: design by mechanochemistry

R Schlem, CF Burmeister, P Michalowski… - Advanced Energy …, 2021 - Wiley Online Library
Commercialization of solid‐state batteries requires the upscaling of the material syntheses
as well as the mixing of electrode composites containing the solid electrolyte, cathode active …

Influence of crystallinity of lithium thiophosphate solid electrolytes on the performance of solid‐state batteries

S Wang, W Zhang, X Chen, D Das… - Advanced Energy …, 2021 - Wiley Online Library
Solid electrolytes (SEs) largely define the properties of all‐solid‐state batteries (ASSBs) and
are expected to improve their safety, stability, and performance. Their ionic conductivity has …

Linking solid electrolyte degradation to charge carrier transport in the thiophosphate‐based composite cathode toward solid‐state lithium‐sulfur batteries

S Ohno, C Rosenbach, GF Dewald… - Advanced Functional …, 2021 - Wiley Online Library
Solid‐state lithium‐sulfur batteries (SSLSBs) have the potential to cause a paradigm shift in
energy storage. The use of emerging highly‐conductive solid electrolytes enables high …

Processing strategies to improve cell-level energy density of metal sulfide electrolyte-based all-solid-state li metal batteries and beyond

D Cao, Y Zhao, X Sun, A Natan, Y Wang… - ACS Energy …, 2020 - ACS Publications
All-solid-state Li metal batteries (ASLBs) have the potential to surpass the energy density of
commercial Li ion batteries and improve safety. However, most reported ASLBs deliver …