Progress and prospects in nonlinear extreme-ultraviolet and X-ray optics and spectroscopy

M Chergui, M Beye, S Mukamel, C Svetina… - Nature Reviews …, 2023 - nature.com
Free-electron lasers and high-harmonic-generation table-top systems are new sources of
extreme-ultraviolet to hard X-ray photons, providing ultrashort pulses that are intense …

Reinvented: An Attosecond Chemist

SR Leone - Annual Review of Physical Chemistry, 2023 - annualreviews.org
Attosecond science requires a substantial rethinking of how to make measurements on very
short timescales; how to acquire the necessary equipment, technology, and personnel; and …

Probing matter with nonlinear spectroscopy

SR Leone, DM Neumark - Science, 2023 - science.org
In the Bohr model of the atom, the nominal orbiting period for a 1s electron in the hydrogen
atom is 150 as (1 as= 10− 18 s). Attosecond light pulses are thus in principle short enough to …

Probing electron and hole colocalization by resonant four-wave mixing spectroscopy in the extreme ultraviolet

H Rottke, RY Engel, D Schick, JO Schunck… - Science …, 2022 - science.org
Extending nonlinear spectroscopic techniques into the x-ray domain promises unique
insight into photoexcited charge dynamics, which are of fundamental and applied interest …

[HTML][HTML] Characterizing coherences in chemical dynamics with attosecond time-resolved x-ray absorption spectroscopy

Y Kobayashi, SR Leone - The Journal of Chemical Physics, 2022 - pubs.aip.org
Coherence can drive wave-like motion of electrons and nuclei in photoexcited systems,
which can yield fast and efficient ways to exert materials' functionalities beyond the …

X-ray/extreme ultraviolet floquet state multidimensional spectroscopy, an analogue of multiple quantum nuclear magnetic resonance

JC Wright, DD Kohler, U Bergmann - The journal of physical …, 2023 - ACS Publications
There is great interest in developing fully coherent multidimensional X-ray/extreme
ultraviolet (XUV) spectroscopic techniques because of their capability for achieving atomic …

Simulating strong-field electron-hole dynamics in solids probed by attosecond transient absorption spectroscopy

SM Cavaletto, LB Madsen - Physical Review A, 2024 - APS
We investigate the ultrafast electron dynamics of a model of a wide-band-gap material with
inner, valence, and conduction bands excited by an intense few-femtosecond pump and …

[HTML][HTML] Attosecond absorption and reflection spectroscopy of solids

N Di Palo, G Inzani, GL Dolso, M Talarico, S Bonetti… - APL Photonics, 2024 - pubs.aip.org
Since their introduction, all-optical spectroscopy techniques based on attosecond radiation
have gained the attention of the scientific community because of their energy and time …

Multidimensional high-harmonic echo spectroscopy: Resolving coherent electron dynamics in the EUV regime

S Jiang, M Gudem, M Kowalewski… - Proceedings of the …, 2024 - National Acad Sciences
We theoretically propose a multidimensional high-harmonic echo spectroscopy technique
which utilizes strong optical fields to resolve coherent electron dynamics spanning an …

Extracting doubly excited state lifetimes in helium directly in the time domain with attosecond noncollinear four-wave-mixing spectroscopy

P Rupprecht, NG Puskar, DM Neumark… - Physical Review Research, 2024 - APS
The helium atom, with one nucleus and two electrons, is a prototypical system to study
quantum many-body dynamics. Doubly excited states, or quantum states in which both …