Intrinsically self-healing polymers: from mechanistic insight to current challenges

B Li, PF Cao, T Saito, AP Sokolov - Chemical Reviews, 2022 - ACS Publications
Self-healing materials open new prospects for more sustainable technologies with improved
material performance and devices' longevity. We present an overview of the recent …

Cellulose and the role of hydrogen bonds: not in charge of everything

M Wohlert, T Benselfelt, L Wågberg, I Furó… - Cellulose, 2022 - Springer
In the cellulose scientific community, hydrogen bonding is often used as the explanation for
a large variety of phenomena and properties related to cellulose and cellulose based …

Extremely strong and tough biodegradable poly (urethane) elastomers with unprecedented crack tolerance via hierarchical hydrogen‐bonding interactions

R Guo, Q Zhang, Y Wu, H Chen, Y Liu… - Advanced …, 2023 - Wiley Online Library
The elastomers with the combination of high strength and high toughness have always been
intensively pursued due to their diverse applications. Biomedical applications frequently …

[HTML][HTML] Chemical syntheses of bioinspired and biomimetic polymers toward biobased materials

MS Ganewatta, Z Wang, C Tang - Nature Reviews Chemistry, 2021 - nature.com
The rich structures and hierarchical organizations in nature provide many sources of
inspiration for advanced material designs. We wish to recapitulate properties such as high …

Multiscale toughening mechanisms in biological materials and bioinspired designs

W Huang, D Restrepo, JY Jung, FY Su, Z Liu… - Advanced …, 2019 - Wiley Online Library
Biological materials found in Nature such as nacre and bone are well recognized as light‐
weight, strong, and tough structural materials. The remarkable toughness and damage …

[HTML][HTML] Nanofibrils in nature and materials engineering

S Ling, DL Kaplan, MJ Buehler - Nature Reviews Materials, 2018 - nature.com
Nanofibrillar materials, such as cellulose, chitin and silk, are highly ordered architectures,
formed through the self-assembly of repetitive building blocks into higher-order structures …

Biopolymer nanofibrils: Structure, modeling, preparation, and applications

S Ling, W Chen, Y Fan, K Zheng, K Jin, H Yu… - Progress in polymer …, 2018 - Elsevier
Biopolymer nanofibrils exhibit exceptional mechanical properties with a unique combination
of strength and toughness, while also presenting biological functions that interact with the …

Silk fibroin/hydroxyapatite composites for bone tissue engineering

M Farokhi, F Mottaghitalab, S Samani… - Biotechnology …, 2018 - Elsevier
Silk fibroin (SF) is a natural fibrous polymer with strong potential for many biomedical
applications. SF has attracted interest in the field of bone tissue engineering due to its …

Structures, mechanical properties and applications of silk fibroin materials

LD Koh, Y Cheng, CP Teng, YW Khin, XJ Loh… - Progress in Polymer …, 2015 - Elsevier
For centuries, Bombyx mori silkworm silk fibroin has been used as a high-end textile fiber.
Beyond textiles, silk fibroin has also been used as a surgical suture material for decades …

Moisture sensitive smart yarns and textiles from self‐balanced silk fiber muscles

T Jia, Y Wang, Y Dou, Y Li… - Advanced Functional …, 2019 - Wiley Online Library
Smart textiles that sense, interact, and adapt to environmental stimuli have provided exciting
new opportunities for a variety of applications. However, current advances have largely …