Multiscale CO2 Electrocatalysis to C2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication

T Yan, X Chen, L Kumari, J Lin, M Li, Q Fan… - Chemical …, 2023 - ACS Publications
Electrosynthesis of value-added chemicals, directly from CO2, could foster achievement of
carbon neutral through an alternative electrical approach to the energy-intensive …

Gas diffusion electrodes and membranes for CO2 reduction electrolysers

EW Lees, BAW Mowbray, FGL Parlane… - Nature Reviews …, 2022 - nature.com
The CO2 reduction reaction (CO2RR) is a potential means of using renewable electricity to
synthesize commodity chemicals and fuels. The CO2RR can be performed at industrially …

High carbon utilization in CO2 reduction to multi-carbon products in acidic media

Y Xie, P Ou, X Wang, Z Xu, YC Li, Z Wang, JE Huang… - Nature Catalysis, 2022 - nature.com
Renewable electricity-powered CO2 reduction to multi-carbon (C2+) products offers a
promising route to realization of low-carbon-footprint fuels and chemicals. However, a major …

Surface passivation for highly active, selective, stable, and scalable CO2 electroreduction

J Zhu, J Li, R Lu, R Yu, S Zhao, C Li, L Lv, L Xia… - Nature …, 2023 - nature.com
Electrochemical conversion of CO2 to formic acid using Bismuth catalysts is one the most
promising pathways for industrialization. However, it is still difficult to achieve high formic …

Conversion of CO2 to multicarbon products in strong acid by controlling the catalyst microenvironment

Y Zhao, L Hao, A Ozden, S Liu, RK Miao, P Ou… - Nature …, 2023 - nature.com
Electrosynthesis of multicarbon products from the reduction of CO2 in acidic electrolytes is a
promising approach to overcoming CO2 reactant loss in alkaline and neutral electrolytes; …

Electroreduction of CO2: Advances in the Continuous Production of Formic Acid and Formate

K Fernández-Caso, G Díaz-Sainz… - ACS Energy …, 2023 - ACS Publications
The study of the electrochemical CO2 reduction to obtain formate (HCOO–) or formic acid
(HCOOH) is receiving much attention as a promising technology. Since continuous–mode …

Membrane Electrode Assembly for Electrocatalytic CO2 Reduction: Principle and Application

Z Zhang, X Huang, Z Chen, J Zhu… - Angewandte …, 2023 - Wiley Online Library
Electrocatalytic CO2 reduction reaction (CO2RR) in membrane electrode assembly (MEA)
systems is a promising technology. Gaseous CO2 can be directly transported to the cathode …

CO2 electrolysis to multicarbon products in strong acid

JE Huang, F Li, A Ozden, A Sedighian Rasouli… - Science, 2021 - science.org
Carbon dioxide electroreduction (CO2R) is being actively studied as a promising route to
convert carbon emissions to valuable chemicals and fuels. However, the fraction of input …

Electrochemical CO2 reduction (CO2RR) to multi-carbon products over copper-based catalysts

AR Woldu, Z Huang, P Zhao, L Hu, D Astruc - Coordination Chemistry …, 2022 - Elsevier
Copper has been recognized as the only heterogeneous catalyst leading to the formation of
various products of hydrocarbons and oxygenates, such as ethanol and ethylene, from the …

Bipolar membrane electrolyzers enable high single-pass CO2 electroreduction to multicarbon products

K Xie, RK Miao, A Ozden, S Liu, Z Chen… - Nature …, 2022 - nature.com
In alkaline and neutral MEA CO2 electrolyzers, CO2 rapidly converts to (bi) carbonate,
imposing a significant energy penalty arising from separating CO2 from the anode gas …