Force-triggered rapid microstructure growth on hydrogel surface for on-demand functions

Q Mu, K Cui, ZJ Wang, T Matsuda, W Cui… - Nature …, 2022 - nature.com
Living organisms share the ability to grow various microstructures on their surface to achieve
functions. Here we present a force stamp method to grow microstructures on the surface of …

Probing the molecular mechanism of viscoelastic relaxation in transient networks

S Michida, U Chung, T Katashima - Gels, 2023 - mdpi.com
Hydrogels, which have polymer networks through supramolecular and reversible
interactions, exhibit various mechanical responsibilities to its surroundings. The influence of …

The application of computer simulation in biomedical hydrogels research: A review

Q Liao, S Kong, L Lin, R Tang, Y Luo, S Fu… - Journal of Molecular …, 2024 - Elsevier
Hydrogels, which are intricate reticulated structures formed by the interaction of polymer
chains dispersed in an aqueous solution, have a wide range of biomedicine applications …

Mixed diffusion and relaxation kinetics model for hydrogels swelling

N Yavari, S Azizian - Journal of Molecular Liquids, 2022 - Elsevier
Hydrogels have a unique ability to retain moisture due to the three-dimensional (3D)
polymeric network. Both swelling capacity and swelling rate of hydrogels depend on the …

All-Atom Molecular Dynamics Simulations of Poly (ethylene glycol) Networks in Water for Evaluating Negative Energetic Elasticity

K Hagita, S Nagahara, T Murashima, T Sakai… - …, 2023 - ACS Publications
We performed all-atom molecular dynamics simulations on poly (ethylene glycol)(PEG)
hydrogels to microscopically confirm the recently discovered “negative energetic …

Preparation of a silk fibroin/gelatin composite hydrogel for high-selectively adsorbing bovine hemoglobin

JP Fan, ZT Lai, DY Mao, CF Xie, HP Chen… - Colloids and Surfaces A …, 2023 - Elsevier
Hydrogels are widely used in biomedical applications and separation of biomolecules.
However, they either share limited biocompatibility or possess poor mechanical properties …

Side‐Chain Engineered P Or N‐Type Nonaqueous Polymeric Ionic Gels for Sustainable Ionic Thermoelectrics

S Kim, M Ham, J Lee, J Kim, H Lee… - Advanced Functional …, 2023 - Wiley Online Library
Although ionic hydrogels have been developed recently for innovative wearable electronics,
they necessitate high humidity to diffuse ions in water and fast self‐healing, which negatively …

Solvent-induced negative energetic elasticity in a lattice polymer chain

NC Shirai, N Sakumichi - Physical Review Letters, 2023 - APS
The negative internal energetic contribution to the elastic modulus (negative energetic
elasticity) has been recently observed in polymer gels. This finding challenges the …

Solvable toy model of negative energetic elasticity

A Iwaki, S Ozaki - Physical Review E, 2024 - APS
Recent experiments have established negative energetic elasticity, the negative contribution
of energy to the elastic modulus, as a universal property of polymer gels. To reveal the …

On the origin of the negative energy-related contribution to the elastic modulus of rubber-like gels

LKR Duarte, LG Rizzi - The European Physical Journal E, 2023 - Springer
We consider a coarse-grained polymer model in order to investigate the origin of a recently
discovered negative energy-related contribution to the elastic modulus G (T) of rubber-like …