From femtoseconds to hours—measuring dynamics over 18 orders of magnitude with coherent x-rays

F Lehmkühler, W Roseker, G Grübel - Applied Sciences, 2021 - mdpi.com
X-ray photon correlation spectroscopy (XPCS) enables the study of sample dynamics
between micrometer and atomic length scales. As a coherent scattering technique, it …

X-ray-based techniques to study the nano–bio interface

C Sanchez-Cano, RA Alvarez-Puebla, JM Abendroth… - ACS …, 2021 - ACS Publications
X-ray-based analytics are routinely applied in many fields, including physics, chemistry,
materials science, and engineering. The full potential of such techniques in the life sciences …

Emergence of anomalous dynamics in soft matter probed at the European XFEL

F Lehmkühler, F Dallari, A Jain… - Proceedings of the …, 2020 - National Acad Sciences
Dynamics and kinetics in soft matter physics, biology, and nanoscience frequently occur on
fast (sub) microsecond but not ultrafast timescales which are difficult to probe …

Real-time swelling-collapse kinetics of nanogels driven by XFEL pulses

F Dallari, I Lokteva, J Möller, W Roseker, C Goy… - Science …, 2024 - science.org
Stimuli-responsive polymers are an important class of materials with many applications in
nanotechnology and drug delivery. The most prominent one is poly-N-isopropylacrylamide …

Nonuniform flow dynamics probed by nanosecond x-ray speckle visibility spectroscopy

Y Sun, G Carini, M Chollet, FJ Decker, M Dunne… - Physical Review Letters, 2021 - APS
We report observations of nanosecond nonuniform colloidal dynamics in a free flowing
liquid jet using ultrafast x-ray speckle visibility spectroscopy. Utilizing a nanosecond double …

[PDF][PDF] Nanosecond X-ray photon correlation spectroscopy using pulse time structure of a storage-ring source

W Jo, F Westermeier, R Rysov, O Leupold, F Schulz… - IUCrJ, 2021 - journals.iucr.org
X-ray photon correlation spectroscopy (XPCS) is a routine technique to study slow dynamics
in complex systems at storage-ring sources. Achieving nanosecond time resolution with the …

Glass-liquid and glass-gel transitions of soft-shell particles

L Frenzel, M Dartsch, GM Balaguer, F Westermeier… - Physical Review E, 2021 - APS
We study the structure and dynamics of colloidal particles with a spherical hard core and a
thermo-responsive soft shell over the whole phase diagram by means of small-angle x-ray …

Performance of a cryo-cooled crystal monochromator illuminated by hard X-rays with MHz repetition rate at the European X-ray Free-Electron Laser

I Petrov, U Boesenberg, VA Bushuev, J Hallmann… - Optics …, 2022 - opg.optica.org
Due to the high intensity and MHz repetition rate of photon pulses generated by the
European X-ray Free-Electron Laser, the heat load on silicon crystal monochromators can …

The phase diagram of colloidal silica–PNIPAm core–shell nanogels

L Frenzel, F Lehmkühler, M Koof, I Lokteva, G Grübel - Soft Matter, 2020 - pubs.rsc.org
We study the structure and dynamics of aqueous dispersions of densely packed core–shell
nanoparticles composed of a silica core and a poly (N-isoproylacrylamide)(PNIPAm) shell …

Single and multi-pulse based X-ray photon correlation spectroscopy

W Jo, S Stern, F Westermeier, R Rysov, M Riepp… - Optics express, 2023 - opg.optica.org
The ability of pulsed nature of synchrotron radiation opens up the possibility of studying
microsecond dynamics in complex materials via speckle-based techniques. Here, we …