Relationship between Energetic Disorder and Reduced Recombination of Free Carriers in Organic Solar Cells

SM Hosseini, S Wilken, B Sun, F Huang… - Advanced Energy …, 2023 - Wiley Online Library
Reducing non‐radiative recombination is key to achieve high fill factors (FFs) in organic
solar cells. While it is generally accepted that recombination proceeds via charge transfer …

materials and modelling for organic photovoltaic devices

O Doat, BH Barboza, A Batagin‐Neto… - Polymer …, 2022 - Wiley Online Library
This review gives a simple and pedagogical introduction to the field of materials and their
modelling for the active layer in organic photovoltaic devices. It gives a perspective on past …

Computational chemistry advances on benzodithiophene-based organic photovoltaic materials

FA Angel, MB Camarada, IA Jessop - Critical Reviews in Solid …, 2023 - Taylor & Francis
Over the past years, highly efficient conjugated polymers and small molecules have led to
the development of organic photovoltaics (OPVs) as a promising alternative to conventional …

Jumping kinetic Monte Carlo: Fast and accurate simulations of partially delocalized charge transport in organic semiconductors

JT Willson, W Liu, D Balzer, I Kassal - The Journal of Physical …, 2023 - ACS Publications
Developing devices using disordered organic semiconductors requires accurate and
practical models of charge transport. In these materials, charge transport occurs through …

How to reduce charge recombination in organic solar cells: There are still lessons to learn from P3HT: PCBM

S Wilken, D Scheunemann, S Dahlström… - Advanced Electronic …, 2021 - Wiley Online Library
Suppressing charge recombination is key for organic solar cells to become commercial
reality. However, there is still no conclusive picture of how recombination losses are …

Slow relaxation of photogenerated charge carriers boosts open-circuit voltage of organic solar cells

T Upreti, S Wilken, H Zhang… - The Journal of Physical …, 2021 - ACS Publications
Among the parameters determining the efficiency of an organic solar cell, the open-circuit
voltage (V OC) is the one with most room for improvement. Existing models for the …

The role of delocalization and excess energy in the quantum efficiency of organic solar cells and the validity of optical reciprocity relations

N Felekidis, A Melianas… - The journal of physical …, 2020 - ACS Publications
The photon energy dependence of long-range charge separation is studied for two
prototypical polymer: fullerene systems. The internal quantum efficiency (IQE) of PCDTBT …

On the device physics of high‐efficiency ternary solar cells

T Upreti, Y Wang, F Gao, M Kemerink - Solar RRL, 2022 - Wiley Online Library
Mixing a third compound into the active layer of an organic bulk heterojunction solar cell to
form a ternary system has become an established way to improve performance. Various …

General rules for the impact of energetic disorder and mobility on nongeminate recombination in phase-separated organic solar cells

G Zuo, S Shoaee, M Kemerink, D Neher - Physical Review Applied, 2021 - APS
State-of-the-art organic solar cells exhibit power conversion efficiencies of 18% and above.
These devices benefit from the suppression of free charge recombination with regard to the …

From Molecules to Devices: A Multiscale Approach to Evaluating Organic Photovoltaics

K Patrikar, K Patadia, R Khatua… - Journal of Chemical …, 2024 - ACS Publications
Due to their efficient molecular design, nonfullerene acceptors (NFAs) have significantly
advanced organic photovoltaics (OPVs). However, the lack of models to screen and …