Reaction Environment Regulation for Electrocatalytic CO2 Reduction in Acids

M Zeng, W Fang, Y Cen, X Zhang, Y Hu… - Angewandte …, 2024 - Wiley Online Library
The electrocatalytic CO2 reduction reaction (CO2RR) is a sustainable route for converting
CO2 into value‐added fuels and feedstocks, advancing a carbon‐neutral economy. The …

Addressing the Carbonate Issue: Electrocatalysts for Acidic CO2 Reduction Reaction

W Wu, L Xu, Q Lu, J Sun, Z Xu, C Song… - Advanced …, 2024 - Wiley Online Library
Electrochemical CO2 reduction reaction (CO2RR) powered by renewable energy provides a
promising route to CO2 conversion and utilization. However, the widely used …

Steering the Selectivity of Carbon Dioxide Electroreduction from Single-Carbon to Multicarbon Products on Metal–Organic Frameworks via Facet Engineering

P Lu, J Lv, Y Chen, Y Ma, Y Wang, W Lyu, J Yu… - Nano Letters, 2024 - ACS Publications
Although metal–organic frameworks (MOFs) have attracted more attention for the
electrocatalytic CO2 reduction reaction (CO2RR), obtaining multicarbon products with a high …

Efficient acidic CO2 electroreduction to formic acid by modulating electrode structure at industrial-level current

Z Wang, H Li, T Dong, Y Geng, X Tian, R Chang… - Chemical Engineering …, 2024 - Elsevier
Acidic CO 2 electroreduction has the potential to synthesize low carbon footprint chemicals
using renewable electricity. However, proton-rich environments can lead to strong hydrogen …

Targeted CO bond cleavage of* CH2CHO at copper active sites for efficient electrosynthesis of ethylene from CO2 reduction

H Zhang, X Wang, Y Sun, X Wang, Z Tang, S Li… - Applied Catalysis B …, 2024 - Elsevier
CH 2 CHO, a pivotal intermediate in CO 2 reduction reaction (CO 2 RR) on copper-based
catalysts, hinges on the strength of Cu-C and CO bonds for the selective production of …

Modulating Interfacial Hydrogen-Bond Environment by Electrolyte Engineering Promotes Acidic CO2 Electrolysis

W Ge, L Dong, C Wang, Y Zhu, Z Liu, H Jiang… - ACS Catalysis, 2024 - ACS Publications
Acidic CO2 electroreduction offers a promising strategy for achieving a high CO2 utilization
efficiency. However, it is highly challenging to inhibit the competing hydrogen evolution …

Integrated carbon capture and CO production from bicarbonates through bipolar membrane electrolysis

H Song, CA Fernández, H Choi, PW Huang… - Energy & …, 2024 - pubs.rsc.org
The electrochemical CO2 reduction reaction (CO2RR) offers an environmentally friendly
method to transform sequestered CO2. While gas-phase electrolysis systems provide high …

Operando Observation of (Bi)carbonate Precipitation during Electrochemical CO2 Reduction in Strongly Acidic Electrolytes

F Bernasconi, N Plainpan, M Mirolo, Q Wang… - Acs …, 2024 - ACS Publications
Precipitation of (bi) carbonate salts during the electrochemical CO2 reduction (CO2RR) has
been identified as a major cause of degradation and one of the main challenges to be …

Enhancing Carbon Efficiency in Electrochemical CO2 Reduction at Silver Gas Diffusion Electrodes–The Effect of Acidic Electrolytes Explained via TFFA Modeling

M Löffelholz, J Osiewacz, L Weseler… - Journal of The …, 2023 - iopscience.iop.org
Recently, there has been a growing focus on enhancing carbon efficiency in the field of
electrochemical CO 2 reduction, quantifying the proportion of CO 2 converted …

Structure-induced interfacial activation convoying the CO-relayed conversion of CO2 to dimethyl carbonate

SG Han, S Zhou, X Li, J Zhao, WB Wei, L Zheng… - Chemical Engineering …, 2024 - Elsevier
The recognition of structure-induced interfacial activation in heterogenized molecule
catalysts is essential to steer CO 2 value-added electroconversion but remains inadequate …