MD Karkas, O Verho, EV Johnston… - Chemical reviews, 2014 - ACS Publications
The sustainable production of clean energy constitutes one of the most important scientific challenges of the 21st century. Currently, the major part of the global energy supply is …
In natural photosynthesis, the light-driven splitting of water into electrons, protons and molecular oxygen forms the first step of the solar-to-chemical energy conversion process …
M Suga, F Akita, M Sugahara, M Kubo, Y Nakajima… - Nature, 2017 - nature.com
Photosystem II (PSII) is a huge membrane-protein complex consisting of 20 different subunits with a total molecular mass of 350 kDa for a monomer. It catalyses light-driven …
M Suga, F Akita, K Hirata, G Ueno, H Murakami… - Nature, 2015 - nature.com
Photosynthesis converts light energy into biologically useful chemical energy vital to life on Earth. The initial reaction of photosynthesis takes place in photosystem II (PSII), a 700 …
O2 formation in photosystem II (PSII) is a vital event on Earth, but the exact mechanism remains unclear. The presently prevailing theoretical model is “radical coupling”(RC) …
Oxygen, which supports all aerobic life, is produced by photosynthetic water oxidation in plants, algae, and cyanobacteria. The water-oxidation reaction probably first appeared in …
Natural photosynthesis stores sunlight in chemical energy carriers, but it has not evolved for the efficient synthesis of fuels, such as H2. Semi-artificial photosynthesis combines the …
Two decades ago, theoretical model calculations played a truly minor role in understanding mechanisms of redox-active metalloenzymes. The methods available to treat transition …
Biological water oxidation, performed by a single enzyme, photosystem II, is a central research topic not only in understanding the photosynthetic apparatus but also for the …