Sensors are perhaps the most important and integral components of our modern society.
With global warming and environmental pollution garnering ever-increasing attention, as …

Heterogeneous and combined hetero-/homogeneous chemical processes have attracted
increased attention in many energy conversion systems, which include large-scale power …

We report the operando imaging of the methyl radical mole fraction above a working
catalyst. Using photofragmentation laser-induced fluorescence (PF-LIF), we imaged methyl …

The effects of the carrier and the content of the active species were studied in the carbon
monoxide oxidation process. MnO x catalysts supported on ZrO 2, CeO 2, MgO, SiO 2, and …

Conspectus Motivated mainly by catalysis, gas–surface interaction between single crystal
surfaces and molecules has been studied for decades. Most of these studies have been …

A direct correlation between the reaction activity and the surface structure of a catalyst is
generally needed to better understand the mechanisms behind the heterogeneous catalysis …

The catalytic oxidation of CO on transition metals, such as Pt, is commonly viewed as a
sharp transition from the CO‐inhibited surface to the active metal, covered with O. However …

Curved crystals are a simple but powerful approach to bridge the gap between single crystal
surfaces and nanoparticle catalysts, by allowing a rational assessment of the role of active …

Many surface science experiments within heterogeneous catalysis are now conducted in
realistic conditions at higher pressures. At these pressures, localized gas conditions will …

Many important chemically reacting systems are inherently multi-dimensional with spatial
and temporal variations in the thermochemical state, which can be strongly coupled to …