Optical spectroscopy and modeling of uranium gas-phase oxidation: Progress and perspectives

EJ Kautz, EN Weerakkody, MS Finko, D Curreli… - … Acta Part B: Atomic …, 2021 - Elsevier
Studies related to U gas-phase oxidation through plasma-and thermo-chemistry are
important for many fields, including environmental monitoring, forensic analysis, debris …

Laser ablation spectrometry for studies of uranium plasmas, reactor monitoring, and spent fuel safety

M Burger, LA Finney, L Garrett, SS Harilal… - … Acta Part B: Atomic …, 2021 - Elsevier
Nuclear security is one of the defining challenges of our time. Nuclear threats range from
deliberate dispersal of radioactive material to contaminate the vital infrastructure to diversion …

[HTML][HTML] Optical spectroscopy of laser-produced plasmas for standoff isotopic analysis

SS Harilal, BE Brumfield, NL LaHaye… - Applied Physics …, 2018 - pubs.aip.org
Rapid, in-field, and non-contact isotopic analysis of solid materials is extremely important to
a large number of applications, such as nuclear nonproliferation monitoring and forensics …

Spectroscopic signatures and oxidation characteristics of nanosecond laser-induced cerium plasmas

EH Kwapis, E Villa-Aleman, KC Hartig - Spectrochimica Acta Part B: Atomic …, 2023 - Elsevier
Improving technologies related to the wide area environmental sampling of nuclear
materials supports the nuclear nonproliferation mission of preventing the proliferation of …

Physical conditions for UO formation in laser-produced uranium plumes

SS Harilal, EJ Kautz, BE Bernacki… - Physical Chemistry …, 2019 - pubs.rsc.org
We investigate the oxidation of uranium (U) species, the physical conditions leading to
uranium monoxide (UO) formation and the interplay between plume hydrodynamics and …

The role of ambient gas confinement, plasma chemistry, and focusing conditions on emission features of femtosecond laser-produced plasmas

EJ Kautz, J Yeak, BE Bernacki, MC Phillips… - Journal of analytical …, 2020 - pubs.rsc.org
Ultrafast laser ablation coupled with optical emission spectroscopy is currently under
development for standoff detection of elements and their isotopes for a wide range of …

The effect of oxygen concentration on the speciation of laser ablated uranium

MA Burton, AW Auner, JC Crowhurst, PS Boone… - Scientific Reports, 2022 - nature.com
In order to model the fate and transport of particles following a nuclear explosion, there must
first be an understanding of individual physical and chemical processes that affect particle …

Time-resolved imaging of atoms and molecules in laser-produced uranium plasmas

EJ Kautz, PJ Skrodzki, M Burger, BE Bernacki… - Journal of Analytical …, 2019 - pubs.rsc.org
Gas-phase oxidation of uranium (U), plume chemistry, and the corresponding impact on
optical emission features of the U plasma are investigated. Plasmas were produced via …

Plume dynamics and gas-phase molecular formation in transient laser-produced uranium plasmas

PJ Skrodzki, M Burger, I Jovanovic, MC Phillips… - Physics of …, 2019 - pubs.aip.org
The dynamics of expansion, thermodynamics, and chemical reactions in laser-produced
plasmas is of general interest for all laser ablation applications. This study investigates the …

Quantitative absorption spectroscopy of laser-produced plasmas

EN Weerakkody, NG Glumac - Journal of Physics D: Applied …, 2021 - iopscience.iop.org
Absorption spectroscopy with a xenon flash lamp source has been used to probe laser-
produced plasmas. Signatures from atomic, ionic, monoxide, monohydride, and mononitride …