Emerging ultrafast techniques for studying quantum materials

A Zong, BR Nebgen, SC Lin, JA Spies… - Nature Reviews …, 2023 - nature.com
In quantum materials, emergent functional properties resulting from strong correlations or
electronic topology offer opportunities for new applications. Over the past decade, ultrafast …

Carriers, quasi-particles, and collective excitations in halide perovskites

J Fu, S Ramesh, JW Melvin Lim, TC Sum - Chemical Reviews, 2023 - ACS Publications
Halide perovskites (HPs) are potential game-changing materials for a broad spectrum of
optoelectronic applications ranging from photovoltaics, light-emitting devices, lasers to …

Confinement and exciton binding energy effects on hot carrier cooling in lead halide perovskite nanomaterials

BP Carwithen, TR Hopper, Z Ge, N Mondal, T Wang… - ACS …, 2023 - ACS Publications
The relaxation of the above-gap (“hot”) carriers in lead halide perovskites (LHPs) is
important for applications in photovoltaics and offers insights into carrier–carrier and carrier …

Transient High-Harmonic Spectroscopy in an Inorganic–Organic Lead Halide Perovskite

MLS van der Geest, JJ de Boer, K Murzyn… - The Journal of …, 2023 - ACS Publications
High-harmonic generation is the frequency upconversion of an intense femtosecond infrared
laser in a material. In condensed-phase high-harmonic generation, laser-driven currents of …

Electronic and structural fingerprints of charge-density-wave excitations in extreme ultraviolet transient absorption spectroscopy

T Heinrich, HT Chang, S Zayko, K Rossnagel, M Sivis… - Physical Review X, 2023 - APS
Femtosecond core-level transient absorption spectroscopy is utilized to investigate
photoinduced dynamics of the charge density wave in 1 T-TiSe 2 at the Ti M 2, 3 edge (32 …

Ultrafast dynamics in perovskite-based optoelectronic devices

S Gong, Y Huang, X Yu, Q Hu, J Liu, J Meng… - Cell Reports Physical …, 2023 - cell.com
Halide-perovskite-based materials are rising stars for optoelectronic applications. The key
for optoelectronic device development is the photogenerated carrier dynamics, which …

Hot carrier extraction from 2D semiconductor photoelectrodes

R Austin, YR Farah, T Sayer… - Proceedings of the …, 2023 - National Acad Sciences
Hot carrier-based energy conversion systems could double the efficiency of conventional
solar energy technology or drive photochemical reactions that would not be possible using …

A-site cation influence on the conduction band of lead bromide perovskites

GJ Man, C Kamal, A Kalinko, D Phuyal… - Nature …, 2022 - nature.com
Hot carrier solar cells hold promise for exceeding the Shockley-Queisser limit. Slow hot
carrier cooling is one of the most intriguing properties of lead halide perovskites and …

Direct observation of ultrafast lattice distortions during exciton–polaron formation in lead halide perovskite nanocrystals

H Seiler, D Zahn, VCA Taylor, MI Bodnarchuk… - ACS …, 2023 - ACS Publications
The microscopic origin of slow hot-carrier cooling in lead halide perovskites remains
debated and has direct implications for applications. Slow hot-carrier cooling of several …

The Hot Phonon Bottleneck Effect in Metal Halide Perovskites

T Faber, L Filipovic, LJA Koster - The Journal of Physical …, 2024 - ACS Publications
The hot phonon bottleneck (HPB) effect has been proposed as one of the main phenomena
behind the slow cooling in metal halide perovskites. Even though consensus has been …