Measuring molecular magnets for quantum technologies

E Moreno-Pineda, W Wernsdorfer - Nature Reviews Physics, 2021 - nature.com
Single-molecule magnets (SMMs) have been proposed for applications in high-density
storage, quantum simulation, quantum computing and spintronics applications. Bulk …

Molecular single-ion magnets based on lanthanides and actinides: Design considerations and new advances in the context of quantum technologies

SG McAdams, AM Ariciu, AK Kostopoulos… - Coordination Chemistry …, 2017 - Elsevier
Over the past fifteen years or so, the study of f-element single-ion magnets (f-SIMs) has gone
from being a sub-discipline of molecular magnetism to an established field of research in its …

Enhancing coherence in molecular spin qubits via atomic clock transitions

M Shiddiq, D Komijani, Y Duan, A Gaita-Ariño… - Nature, 2016 - nature.com
Quantum computing is an emerging area within the information sciences revolving around
the concept of quantum bits (qubits). A major obstacle is the extreme fragility of these qubits …

Spin dynamics in single-molecule magnets and molecular qubits

D Aravena, E Ruiz - Dalton Transactions, 2020 - pubs.rsc.org
Over recent decades, much effort has been made to lengthen spin relaxation/decoherence
times of single-molecule magnets and molecular qubits by following different chemical …

Molecular nanomagnets: a viable path toward quantum information processing?

A Chiesa, P Santini, E Garlatti, F Luis… - Reports on Progress in …, 2024 - iopscience.iop.org
Molecular nanomagnets (MNMs), molecules containing interacting spins, have been a
playground for quantum mechanics. They are characterized by many accessible low-energy …

Tuning of molecular qubits: very long coherence and spin–lattice relaxation times

K Bader, M Winkler, J van Slageren - Chemical Communications, 2016 - pubs.rsc.org
We report a pulsed EPR study on different transition metal phthalocyanines, elucidating the
dependence of spin relaxation on solvent, ligand and metal ion. Coherence times of> 40 µs …

Heterometallic rings: their physics and use as supramolecular building blocks

EJL McInnes, GA Timco, GFS Whitehead… - Angewandte Chemie …, 2015 - Wiley Online Library
An enormous family of heterometallic rings has been made. The first were Cr7M rings where
M= NiII, ZnII, MnII, and rings have been made with as many as fourteen metal centers in the …

Making hybrid [n]-rotaxanes as supramolecular arrays of molecular electron spin qubits

A Fernandez, J Ferrando-Soria, EM Pineda… - Nature …, 2016 - nature.com
Quantum information processing (QIP) would require that the individual units involved—
qubits—communicate to other qubits while retaining their identity. In many ways this …

The rise of single-ion magnets as spin qubits

YS Ding, YF Deng, YZ Zheng - Magnetochemistry, 2016 - mdpi.com
Recent studies revealed that magnetic molecules with single spin centers showed exciting
phenomena related to quantum information processing, such as long quantum coherence …

Modelling Conformational Flexibility in a Spectrally Addressable Molecular Multi‐Qubit Model System

CJ Rogers, D Asthana, A Brookfield… - Angewandte …, 2022 - Wiley Online Library
Dipolar coupled multi‐spin systems have the potential to be used as molecular qubits.
Herein we report the synthesis of a molecular multi‐qubit model system with three …