From femtoseconds to hours—measuring dynamics over 18 orders of magnitude with coherent x-rays

F Lehmkühler, W Roseker, G Grübel - Applied Sciences, 2021 - mdpi.com
X-ray photon correlation spectroscopy (XPCS) enables the study of sample dynamics
between micrometer and atomic length scales. As a coherent scattering technique, it …

Hard x-ray photon correlation spectroscopy methods for materials studies

AR Sandy, Q Zhang, LB Lurio - Annual Review of Materials …, 2018 - annualreviews.org
Understanding and designing sophisticated new materials require measurements of not
only their average structural properties but also their dynamic behavior. X-ray photon …

Phase transition dynamics in a complex oxide heterostructure

Q Zhang, G Hu, V Starchenko, G Wan, EM Dufresne… - Physical Review Letters, 2022 - APS
Understanding the behavior of defects in the complex oxides is key to controlling myriad
ionic and electronic properties in these multifunctional materials. The observation of defect …

Structural dynamics of materials probed by X-ray photon correlation spectroscopy

A Madsen, A Fluerasu, B Ruta - … Light Sources and Free-Electron Lasers …, 2020 - Springer
In this chapter we discuss coherent X-ray scattering, photon statistics of speckle patterns,
and X-ray photon correlation spectroscopy (XPCS). XPCS is a coherent X-ray scattering …

Outlook for artificial intelligence and machine learning at the NSLS-II

SI Campbell, DB Allan, AM Barbour… - Machine Learning …, 2021 - iopscience.iop.org
We describe the current and future plans for using artificial intelligence and machine
learning (AI/ML) methods at the National Synchrotron Light Source II (NSLS-II), a scientific …

Sub-microsecond-resolved multi-speckle X-ray photon correlation spectroscopy with a pixel array detector

Q Zhang, EM Dufresne, S Narayanan… - Journal of …, 2018 - journals.iucr.org
Small-angle X-ray photon correlation spectroscopy (XPCS) measurements spanning delay
times from 826 ns to 52.8 s were performed using a photon-counting pixel array detector …

Dynamic scaling of colloidal gel formation at intermediate concentrations

Q Zhang, D Bahadur, EM Dufresne, P Grybos… - Physical Review Letters, 2017 - APS
We have examined the formation and dissolution of gels composed of intermediate volume-
fraction nanoparticles with temperature-dependent short-range attractions using small-angle …

[PDF][PDF] Ultra-small-angle X-ray photon correlation spectroscopy using the Eiger detector

T Zinn, A Homs, L Sharpnack, G Tinti… - Journal of …, 2018 - journals.iucr.org
Successful implementation of the single-photon-counting Eiger 500k pixel array detector for
sub-millisecond X-ray photon correlation spectroscopy (XPCS) measurements in the ultra …

[PDF][PDF] 20 µs-resolved high-throughput X-ray photon correlation spectroscopy on a 500k pixel detector enabled by data-management workflow

Q Zhang, EM Dufresne, Y Nakaye… - Journal of …, 2021 - journals.iucr.org
The performance of the new 52 kHz frame rate Rigaku XSPA-500k detector was
characterized on beamline 8-ID-I at the Advanced Photon Source at Argonne for X-ray …

[PDF][PDF] Direct measurement of Stokes–Einstein diffusion of Cowpea mosaic virus with 19 µs-resolved XPCS

K Switalski, J Fan, L Li, M Chu, E Sarnello… - Journal of …, 2022 - journals.iucr.org
Brownian motion of Cowpea mosaic virus (CPMV) in water was measured using small-angle
X-ray photon correlation spectroscopy (SA-XPCS) at 19.2 µs time resolution. It was found …