Electrocatalysis for CO 2 conversion: from fundamentals to value-added products

G Wang, J Chen, Y Ding, P Cai, L Yi, Y Li… - Chemical Society …, 2021 - pubs.rsc.org
The continuously increasing CO2 released from human activities poses a great threat to
human survival by fluctuating global climate and disturbing carbon balance among the four …

Stability and Degradation Mechanisms of Copper‐Based Catalysts for Electrochemical CO2 Reduction

S Popović, M Smiljanić, P Jovanovič… - Angewandte …, 2020 - Wiley Online Library
To date, copper is the only monometallic catalyst that can electrochemically reduce CO2 into
high value and energy‐dense products, such as hydrocarbons and alcohols. In recent years …

Atomic-scale surface restructuring of copper electrodes under CO2 electroreduction conditions

R Amirbeigiarab, J Tian, A Herzog, C Qiu… - Nature Catalysis, 2023 - nature.com
Potentiodynamic methods that induce structural changes in Cu catalysts for the
electrochemical reduction of CO2 (CO2RR) have been identified as a promising strategy for …

[HTML][HTML] Cu-Ag tandem catalysts for high-rate CO2 electrolysis toward multicarbons

C Chen, Y Li, S Yu, S Louisia, J Jin, M Li, MB Ross… - Joule, 2020 - cell.com
Tandem electrocatalysis decouples individual steps within a chemically complicated
pathway via multicomponent catalyst design. Such a concept is attractive for CO 2 electro …

Solution-based Cu+ transient species mediate the reconstruction of copper electrocatalysts for CO2 reduction

J Vavra, GPL Ramona, F Dattila, A Kormányos… - Nature Catalysis, 2024 - nature.com
Understanding metal surface reconstruction is of the utmost importance in electrocatalysis,
as this phenomenon directly affects the nature of available active sites. However, its dynamic …

Dynamic transformation of cubic copper catalysts during CO2 electroreduction and its impact on catalytic selectivity

P Grosse, A Yoon, C Rettenmaier, A Herzog… - Nature …, 2021 - nature.com
To rationally design effective and stable catalysts for energy conversion applications, we
need to understand how they transform under reaction conditions and reveal their …

Grain Boundary‐Derived Cu+/Cu0 Interfaces in CuO Nanosheets for Low Overpotential Carbon Dioxide Electroreduction to Ethylene

J Zhang, Y Wang, Z Li, S Xia, R Cai, L Ma… - Advanced …, 2022 - Wiley Online Library
Electrochemical CO2 reduction reaction can be used to produce value‐added hydrocarbon
fuels and chemicals by coupling with clean electrical energy. However, highly active …

Imaging electrochemically synthesized Cu2O cubes and their morphological evolution under conditions relevant to CO2 electroreduction

RM Arán-Ais, R Rizo, P Grosse, G Algara-Siller… - Nature …, 2020 - nature.com
Copper is a widely studied catalyst material for the electrochemical conversion of carbon
dioxide to valuable hydrocarbons. In particular, copper-based nanostructures expressing …

Real‐time Monitoring Reveals Dissolution/Redeposition Mechanism in Copper Nanocatalysts during the Initial Stages of the CO2 Reduction Reaction

J Vavra, TH Shen, D Stoian, V Tileli… - Angewandte …, 2021 - Wiley Online Library
Size, morphology, and surface sites of electrocatalysts have a major impact on their
performance. Understanding how, when, and why these parameters change under …

Shaping Copper Nanocatalysts to Steer Selectivity in the Electrochemical CO2 Reduction Reaction

K Rossi, R Buonsanti - Accounts of Chemical Research, 2022 - ACS Publications
Conspectus The carbon-neutral production of fuels and chemical feedstocks is one of the
grand challenges for our society to solve. The electrochemical conversion of CO2 is …