Cellulose nanofibril nanopapers and bioinspired nanocomposites: a review to understand the mechanical property space

AJ Benítez, A Walther - Journal of Materials Chemistry A, 2017 - pubs.rsc.org
Cellulose nanofibrils (CNFs) emerge as a renewable and sustainable feedstock for future
biobased high-performance materials with environmentally friendly character. They allow for …

A review on the very high nanofiller-content nanocomposites: Their preparation methods and properties with high aspect ratio fillers

J George, H Ishida - Progress in Polymer Science, 2018 - Elsevier
For many years, the inorganic content in nanocomposites has seldom exceeded 10 vol%.
Novel fabrication methods have been employed to incorporate high inorganic loading within …

Humidity and multiscale structure govern mechanical properties and deformation modes in films of native cellulose nanofibrils

AJ Benítez, J Torres-Rendon, M Poutanen… - …, 2013 - ACS Publications
Nanopapers formed by stiff and strong native cellulose nanofibrils are emerging as
mechanically robust and sustainable materials to replace high-performance plastics or as …

Nacre-mimetics with synthetic nanoclays up to ultrahigh aspect ratios

P Das, JM Malho, K Rahimi, FH Schacher… - Nature …, 2015 - nature.com
Nacre-mimetics hold great promise as mechanical high-performance and functional
materials. Here we demonstrate large progress of mechanical and functional properties of …

Self-assembled, iridescent, crustacean-mimetic nanocomposites with tailored periodicity and layered cuticular structure

B Wang, A Walther - ACS nano, 2015 - ACS Publications
Natural high-performance materials inspire the pursuit of ordered hard/soft nanocomposite
structures at high fractions of reinforcements and with balanced molecular interactions …

Self-assembled bioinspired nanocomposites

F Lossada, D Hoenders, J Guo, D Jiao… - Accounts of Chemical …, 2020 - ACS Publications
Conspectus Bioinspired materials engineering impacts the design of advanced functional
materials across many domains of sciences from wetting behavior to optical and mechanical …

Hierarchical nacre mimetics with synergistic mechanical properties by control of molecular interactions in self‐healing polymers

B Zhu, N Jasinski, A Benitez, M Noack… - Angewandte Chemie …, 2015 - Wiley Online Library
Designing the reversible interactions of biopolymers remains a grand challenge for an
integral mimicry of mechanically superior biological composites. Yet, they are the key to …

Toughness and fracture properties in nacre‐mimetic clay/polymer nanocomposites

M Morits, T Verho, J Sorvari, V Liljeström… - Advanced Functional …, 2017 - Wiley Online Library
Nacre inspires researchers by combining stiffness with toughness by its unique
microstructure of aligned aragonite platelets. This brick‐and‐mortar structure of reinforcing …

Bioinspired interface engineering for moisture resistance in nacre-mimetic cellulose nanofibrils/clay nanocomposites

K Yao, S Huang, H Tang, Y Xu… - … Applied Materials & …, 2017 - ACS Publications
The interfacial adhesion design between “mortar” and “bricks” is essential for mechanical
and barrier performance of nanocellulose-based nacre-mimetic nanocomposites, especially …

Exceptionally ductile and tough biomimetic artificial nacre with gas barrier function

A Eckert, T Rudolph, J Guo, T Mang… - Advanced …, 2018 - Wiley Online Library
Synthetic mimics of natural high‐performance structural materials have shown great and
partly unforeseen opportunities for the design of multifunctional materials. For nacre‐mimetic …