Laser-cooled molecules

NJ Fitch, MR Tarbutt - Advances in atomic, molecular, and optical Physics, 2021 - Elsevier
The last few years have seen rapid progress in the application of laser cooling to molecules.
In this review, we examine what kinds of molecules can be laser cooled, how to design a …

Direct laser cooling of polyatomic molecules

BL Augenbraun, L Anderegg, C Hallas… - Advances in Atomic …, 2023 - Elsevier
Over the past decade, tremendous progress has been made to extend the tools of laser
cooling and trapping to molecules. Those same tools have recently been applied to …

Sisyphus laser cooling of a polyatomic molecule

I Kozyryev, L Baum, K Matsuda, BL Augenbraun… - Physical review …, 2017 - APS
We perform magnetically assisted Sisyphus laser cooling of the triatomic free radical
strontium monohydroxide (SrOH). This is achieved with principal optical cycling in the …

Structural and electronic trends of optical cycling centers in polyatomic molecules revealed by microwave spectroscopy of MgCCH, CaCCH, and SrCCH

PB Changala, N Genossar-Dan… - Proceedings of the …, 2023 - National Acad Sciences
The unique optical cycling efficiency of alkaline earth metal–ligand molecules has enabled
significant advances in polyatomic laser cooling and trapping. Rotational spectroscopy is an …

Molecular asymmetry and optical cycling: laser cooling asymmetric top molecules

BL Augenbraun, JM Doyle, T Zelevinsky, I Kozyryev - Physical Review X, 2020 - APS
We present a practical roadmap to achieve optical cycling and laser cooling of asymmetric
top molecules (ATMs). Our theoretical analysis describes how reduced molecular symmetry …

Proposal for laser cooling of complex polyatomic molecules

I Kozyryev, L Baum, K Matsuda, JM Doyle - ChemPhysChem, 2016 - Wiley Online Library
An experimentally feasible strategy for direct laser cooling of polyatomic molecules with six
or more atoms is presented. Our approach relies on the attachment of a metal atom to a …

Laser cooling and trapping molecules

D McCarron - Journal of Physics B: Atomic, Molecular and Optical …, 2018 - iopscience.iop.org
The extension of laser cooling and trapping techniques from atoms to molecules is currently
the subject of intense and growing interest. Molecular laser cooling and trapping offers a …

Laser-coolable polyatomic molecules with heavy nuclei

TA Isaev, AV Zaitsevskii, E Eliav - Journal of Physics B: Atomic …, 2017 - iopscience.iop.org
Recently, a few diatomic and polyatomic molecules have been identified as prospective
systems for Doppler/Sisyphus cooling. Doppler/Sisyphus cooling allows us to decrease the …

Determination of CaOH and CaOCH3 vibrational branching ratios for direct laser cooling and trapping

I Kozyryev, TC Steimle, P Yu, DT Nguyen… - New Journal of …, 2019 - iopscience.iop.org
Alkaline earth monoalkoxide free radicals (MORs) have molecular properties conducive to
direct laser cooling to sub-millikelvin temperatures. Using dispersed laser induced …

Characterizing the fundamental bending vibration of a linear polyatomic molecule for symmetry violation searches

A Jadbabaie, Y Takahashi, NH Pilgram… - New Journal of …, 2023 - iopscience.iop.org
Polyatomic molecules have been identified as sensitive probes of charge-parity violating
and parity violating physics beyond the Standard Model (BSM). For example, many linear …