The simplicity of hard spheres as a model system is deceptive. Although the particles interact solely through volume exclusion, that nevertheless suffices for a wealth of static and …
We start with a few concise definitions of the most important concepts discussed in this entry. Glass transition For molecular liquids, the glass transition denotes a crossover from a …
We perform stringent tests of thermodynamic theories of the glass transition over the experimentally relevant temperature regime for several simulated glass-formers. The swap …
VF Hagh, SR Nagel, AJ Liu… - Proceedings of the …, 2022 - National Acad Sciences
The introduction of transient degrees of freedom into a system can lead to novel material design and training protocols that guide a system into a desired metastable state. In this …
Key to resolving the scientific challenge of the glass transition is to understand the origin of the massive increase in viscosity of liquids cooled below their melting temperature (avoiding …
The Random First Order Transition (RFOT) theory started with the pioneering work of Kirkpatrick, Thirumalai and Wolynes. It leverages methods and advances of the theory of …
swap algorithms can shift the glass transition to lower temperatures, a recent unexplained observation constraining the nature of this phenomenon. Here we show that swap dynamics …
It was recently discovered that SWAP, a Monte Carlo algorithm that involves the exchange of pairs of particles of differing diameters, can dramatically accelerate the equilibration of …
A recent breakthrough in glass science has been the synthesis of ultrastable glasses via physical vapor deposition techniques. These samples display enhanced thermodynamic …