[HTML][HTML] Saloplastics and the polyelectrolyte complex continuum: Advances, challenges and prospects

JK Bediako, ESM Mouele, Y El Ouardi… - Chemical Engineering …, 2023 - Elsevier
Polyelectrolytes (PEs) are macromolecules that possess repeating units of ionizable groups
in addition to counterions. Polyelectrolyte complexes (PECs) emanate from the entropy …

Polyelectrolyte-multivalent molecule complexes: physicochemical properties and applications

SE Herrera, ML Agazzi, E Apuzzo, ML Cortez… - Soft Matter, 2023 - pubs.rsc.org
The complexation of polyelectrolytes with other oppositely charged structures gives rise to a
great variety of functional materials with potential applications in a wide spectrum of …

Polyelectrolyte complex coacervation across a broad range of charge densities

AE Neitzel, YN Fang, B Yu, AM Rumyantsev… - …, 2021 - ACS Publications
Polyelectrolyte complex coacervates of homologous (co) polyelectrolytes with a near-ideally
random distribution of a charged and neutral ethylene oxide comonomer were synthesized …

Supramolecular polyelectrolyte hydrogel based on conjoined double-networks for multifunctional applications

WJ Yang, R Zhang, X Guo, R Ma, Z Liu… - Journal of Materials …, 2022 - pubs.rsc.org
Recently, the skin-biomimetic ionic conductive hydrogels have emerged as a competitive
alternative in soft electronics applications due to their excellent ionic conductivity and good …

Looping-in complexation and ion partitioning in nonstoichiometric polyelectrolyte mixtures

S Friedowitz, J Lou, KP Barker, K Will, Y Xia, J Qin - Science Advances, 2021 - science.org
A wide variety of intracellular membraneless compartments are formed via liquid-liquid
phase separation of charged proteins and nucleic acids. Understanding the stability of these …

Effect of dynamically arrested domains on the phase behavior, linear viscoelasticity and microstructure of hyaluronic acid–chitosan complex coacervates

J Es Sayed, C Caïto, A Arunachalam… - …, 2023 - ACS Publications
Complex coacervates make up a class of versatile materials formed as a result of the
electrostatic associations between oppositely charged polyelectrolytes. It is well-known that …

Effect of solvent quality on the phase behavior of polyelectrolyte complexes

L Li, AM Rumyantsev, S Srivastava, S Meng… - …, 2020 - ACS Publications
The role of polyelectrolyte–solvent interactions, among other non-Coulomb interactions, in
dictating the thermodynamics and kinetics of polyelectrolyte complexation is prominent yet …

Bridging field theory and ion pairing in the modeling of polyelectrolytes and complex coacervation

CE Sing, J Qin - Macromolecules, 2023 - ACS Publications
Complex coacervation is a phase separation phenomenon driven by the electrostatic
attraction between oppositely charged macromolecular species. A recent surge of interest in …

Moderated ionic bonding for water-free recyclable polyelectrolyte complex materials

SGM van Lange, DW Te Brake, G Portale… - Science …, 2024 - science.org
While nature extensively uses electrostatic bonding between oppositely charged polymers
to assemble and stabilize materials, harnessing these interactions in synthetic systems has …

Bioinspired processing: complex coacervates as versatile inks for 3D bioprinting

M Khoonkari, J Es Sayed, M Oggioni… - Advanced …, 2023 - Wiley Online Library
Abstract 3D bioprinting is a powerful fabrication technique in biomedical engineering, which
is currently limited by the number of available materials that meet all physicochemical and …