Laser ablation plasmas and spectroscopy for nuclear applications

EH Kwapis, J Borrero, KS Latty, HB Andrews… - Applied …, 2024 - opg.optica.org
The development of measurement methodologies to detect and monitor nuclear-relevant
materials remains a consistent and significant interest across the nuclear energy …

Laser ablation spectrometry for studies of uranium plasmas, reactor monitoring, and spent fuel safety

M Burger, LA Finney, L Garrett, SS Harilal… - … Acta Part B: Atomic …, 2021 - Elsevier
Nuclear security is one of the defining challenges of our time. Nuclear threats range from
deliberate dispersal of radioactive material to contaminate the vital infrastructure to diversion …

Oxidation in laser-generated metal plumes

EJ Kautz, MC Phillips, A Zelenyuk, SS Harilal - Physics of plasmas, 2022 - pubs.aip.org
The temporal evolution of atoms and molecules in a laser-produced plasma was
investigated using optical emission spectroscopy for several metal targets (ie, Al, Ti, Fe, Zr …

Physical conditions for UO formation in laser-produced uranium plumes

SS Harilal, EJ Kautz, BE Bernacki… - Physical Chemistry …, 2019 - pubs.rsc.org
We investigate the oxidation of uranium (U) species, the physical conditions leading to
uranium monoxide (UO) formation and the interplay between plume hydrodynamics and …

Time-resolved formation of uranium and silicon oxides subsequent to the laser ablation of U3Si2

EN Weerakkody, DG Weisz, J Crowhurst… - … Acta Part B: Atomic …, 2020 - Elsevier
The early-time kinetic behavior of species in a plume produced from laser ablation of U 3 Si
2 in an environment containing 2% O 2 is characterized using time-resolved absorption …

The effect of oxygen concentration on the speciation of laser ablated uranium

MA Burton, AW Auner, JC Crowhurst, PS Boone… - Scientific Reports, 2022 - nature.com
In order to model the fate and transport of particles following a nuclear explosion, there must
first be an understanding of individual physical and chemical processes that affect particle …

Vapor-phase aggregation of cerium oxide nanoparticles in a rapidly cooling plasma

K Rodriguez, B Koroglu, J Hammons… - ACS Earth and Space …, 2022 - ACS Publications
Local conditions, such as temperature and oxygen availability, have a pronounced effect on
the formation and evolution of fallout following a nuclear explosion. While the behavior of …

Experimental investigation of uranium volatility during vapor condensation

B Koroglu, Z Dai, M Finko, MR Armstrong… - Analytical …, 2020 - ACS Publications
The predictive models that describe the fate and transport of radioactive materials in the
atmosphere following a nuclear incident (explosion or reactor accident) assume that …

Influence of Temperature History and Flow Mixing on the Vapor-Phase Speciation of Uranium Oxide Nanoparticles

K Rodriguez, EN Weerakkody, Z Dai… - ACS Earth and Space …, 2023 - ACS Publications
The transport of radioactive material following a nuclear event depends heavily on fallout
characteristics (eg, composition, shape, and size), which in turn are controlled by the …

The influence of cooling rate on condensation of iron, aluminum, and uranium oxide nanoparticles

B Koroglu, M Finko, C Saggese, S Wagnon… - Journal of Aerosol …, 2022 - Elsevier
Fundamental observations of particle size distributions are needed to develop models that
predict the fate and transport of radioactive materials in the atmosphere following a nuclear …