Optical Spin Orientation of Localized Electrons and Holes Interacting with Nuclei in a FA0.9Cs0.1PbI2.8Br0.2 Perovskite Crystal

D Kudlacik, NE Kopteva, M Kotur, DR Yakovlev… - ACS …, 2024 - ACS Publications
Optical orientation of carrier spins by circularly polarized light is the basic concept and tool of
spin physics in semiconductors. We study the optical orientation of electrons and holes in a …

Optical Studies of Doped Two-Dimensional Lead Halide Perovskites: Evidence for Rashba-Split Branches in the Conduction Band

E Lafalce, R Bodin, BW Larson, J Hao, MA Haque… - ACS …, 2024 - ACS Publications
Two-dimensional (2D) hybrid organic/inorganic perovskites are an emerging materials class
for optoelectronic and spintronic applications due to strong excitonic absorption and …

Ab initio Wannier-representation-based calculations of photocurrent in semiconductors and metals

J Xu, H Xiao - Physical Review B, 2024 - APS
We present a general ab initio method based on Wannier functions using the covariant
derivative for simulating the photocurrent in solids. The method is widely applicable to …

Magneto-optical studies of hybrid organic/inorganic perovskite: The case of methyl-ammonium lead bromide

UN Huynh, R Bodin, X Pan, P Bailey, H Liu, S McGill… - Physical Review B, 2024 - APS
Picosecond time-resolved and cw magneto-optical methods have been used for studying
the spin-related properties of excitons and photocarriers in methyl-ammonium lead bromide …

Spin Dynamics in Hybrid Halide Perovskites-Effect of Dynamical and Permanent Symmetry Breaking

K Li, J Xu, UN Huynh, R Bodin, M Gupta… - The Journal of …, 2024 - ACS Publications
The hybrid organic–inorganic halide perovskite (HOIP), for example, MAPbBr3, exhibits
extended spin lifetime and apparent spin lifetime anisotropy in experiments. The underlying …

First-principles computational methods for quantum defects in two-dimensional materials: A perspective

H Seo, V Ivády, Y Ping - Applied Physics Letters, 2024 - pubs.aip.org
Quantum defects are atomic defects in materials that provide resources to construct quantum
information devices such as single-photon emitters and spin qubits. Recently, two …

Spin relaxation in graphite due to spin-orbit–phonon interaction from a first-principles density matrix approach

J Xu - Physical Review B, 2024 - APS
We predict intrinsic spin relaxation times (T 1) of graphite due to spin-orbit–phonon
interaction, ie, spin-phonon interaction caused by spin-orbit coupling and electron-phonon …

Decoherence of solid-state spin qubits: a computational perspective

M Onizhuk, G Galli - arXiv preprint arXiv:2405.18535, 2024 - arxiv.org
The usefulness of solid-state spins in quantum technologies depends on how long they can
remain in a coherent superposition of quantum states. This Colloquium discusses how first …

Efficient spin accumulation carried by slow relaxons in chiral tellurium

E Barts, K Tenzin, J Sławińska - arXiv preprint arXiv:2407.01187, 2024 - arxiv.org
Efficient conversion between charge currents and spin signals is crucial for realizing magnet-
free spintronic devices. However, the strong spin-orbit coupling that enables such a …

Electrically Switchable Circular Photogalvanic Effect in Methylammonium Lead Iodide Microcrystals

Y Zhu, Z Song, RB Silva, BM Wang… - arXiv preprint arXiv …, 2024 - arxiv.org
We investigate the circular photogalvanic effect (CPGE) in single-crystalline
methylammonium lead iodide microcrystals under a static electric field. The external electric …