Unraveling the structure and dynamics of excitons in semiconductor quantum dots

P Kambhampati - Accounts of chemical research, 2011 - ACS Publications
The quantum dot, one of the central materials in nanoscience, is a semiconductor crystal
with a physical size on the nanometer length scale. It is often called an “artificial atom” …

Unraveling the excitonics of light emission from metal-halide perovskite quantum dots

P Kambhampati - Nanoscale, 2024 - pubs.rsc.org
Metal halide semicondictor perovskites have been under intense investigation for their
promise in light absorptive applications like photovoltaics. They have more recently …

Bright and grey states in CdSe-CdS nanocrystals exhibiting strongly reduced blinking

P Spinicelli, S Buil, X Quelin, B Mahler, B Dubertret… - Physical review …, 2009 - APS
When compared to standard colloidal nanocrystals, individual CdSe-CdS core-shell
nanocrystals with thick shells exhibit strongly reduced blinking. Analyzing the photon …

Direct observation of higher multiexciton formation and annihilation in CdSe quantum dots

DP Strandell, A Ghosh, D Zenatti… - The Journal of …, 2023 - ACS Publications
Most experiments on multiexcitons (MX) in quantum dots focused on the biexciton (XX),
which is now well-understood. In contrast, there is little understanding of higher MX in …

Light Emission from CsPbBr3 Metal Halide Perovskite Nanocrystals Arises from Dual Emitting States with Distinct Lattice Couplings

DP Strandell, P Kambhampati - Nano Letters, 2023 - ACS Publications
Metal halide perovskite nanocrystals are under intense investigation for their outstanding
optical and electronic properties. The presence of higher fine structure states, let alone …

Challenge to the charging model of semiconductor-nanocrystal fluorescence intermittency from off-state quantum yields and multiexciton blinking

J Zhao, G Nair, BR Fisher, MG Bawendi - Physical review letters, 2010 - APS
Semiconductor nanocrystals emit light intermittently; ie, they “blink,” under steady
illumination. The dark periods have been widely assumed to be due to photoluminescence …

Multiexcitons in type-II colloidal semiconductor quantum dots

D Oron, M Kazes, U Banin - Physical Review B—Condensed Matter and …, 2007 - APS
The spectroscopy and dynamics of multiple excitations on colloidal type-II Cd Te∕ Cd Se
core-shell quantum dots (QDs) are explored via quasi-cw multiexciton spectroscopy. The …

Carrier multiplication yields of and nanocrystals by transient photoluminescence spectroscopy

G Nair, MG Bawendi - Physical Review B—Condensed Matter and Materials …, 2007 - APS
Engineering semiconductors to enhance carrier multiplication (CM) could lead to increased
photovoltaic cell performance and a significant widening of the materials range suitable for …

State-resolved studies of biexcitons and surface trapping dynamics in semiconductor quantum dots

SL Sewall, RR Cooney, KEH Anderson… - The Journal of …, 2008 - pubs.aip.org
Biexcitons in strongly confined, colloidal CdSe quantum dots were investigated with
excitonic state selectivity combined with 10 fs temporal precision. Within the first 50 fs, the …

Heralded spectroscopy reveals exciton–exciton correlations in single colloidal quantum dots

G Lubin, R Tenne, AC Ulku, IM Antolovic, S Burri… - Nano …, 2021 - ACS Publications
Multiply excited states in semiconductor quantum dots feature intriguing physics and play a
crucial role in nanocrystal-based technologies. While photoluminescence provides a natural …