Recent developments in X-ray free-electron lasers have enabled a novel site-selective
probe of coupled nuclear and electronic dynamics in photoexcited molecules, time-resolved …

We present an overview of experimental and theoretical investigations exploring the
dynamical evolution of Rydberg-to-valence character in the electronically excited states of …

We have observed details of the internal motion and dissociation channels in photoexcited
carbon disulfide (CS 2) using time-resolved x-ray scattering (TRXS). Photoexcitation of gas …

We probe the dynamics of dissociating CS 2 molecules across the entire reaction pathway
upon excitation. Photoelectron spectroscopy measurements using laboratory-generated …

An inversion method for time-resolved data from ultrafast experiments is introduced, based
on forward-optimization in a trajectory basis. The method is applied to experimental data …

Time-resolved photoelectron imaging (TRPEI) is a highly differential technique for the
detailed study of non-adiabatic energy redistribution dynamics operating in the electronically …

We studied nonadiabatic dissociation of CS2 from the 1B2 (1Σu+) state using ultrafast
extreme ultraviolet photoelectron spectroscopy. A deep UV (200 nm) laser using the …

The photodissociation dynamics of UV excited CS 2 are investigated using time-resolved
Auger–Meitner (AM) spectroscopy. AM decay is initiated by inner-shell ionisation with a …

Single‐photon ionisation of enantiopure methyl p‐tolyl sulfoxide by circularly polarised light
at 133 nm shows remarkably strong photoelectron circular dichroism (PECD), which has …

Femtosecond pulses of light in the vacuum ultraviolet (VUV) spectral region permit extended
observation of non-adiabatic dynamics in gas-phase molecules. When used as a probe in …