[HTML][HTML] Recent progress in probing atomic and molecular quantum coherence with scanning tunneling microscopy

L Bi, K Liang, G Czap, H Wang, K Yang, S Li - Progress in Surface Science, 2023 - Elsevier
Quantum coherent physics and chemistry concern the creation and manipulation of an
excited-state manifold that contains the superposition and entanglement of multiple quantum …

Imaging surfaces at the space–time limit: New perspectives of time-resolved scanning tunneling microscopy for ultrafast surface science

M Müller - Progress in Surface Science, 2024 - Elsevier
Many fundamental processes in nature occur on ultrashort time scales within picoseconds to
attoseconds, and on intrinsic length scales from nanometers to picometers. The structure of …

Open questions in attochemistry

F Calegari, F Martin - Communications Chemistry, 2023 - nature.com
Attosecond science is nowadays a well-established research field, and table-top attosecond
sources based on high-harmonic generation are routinely used to access electronic motion …

Subcycle mid-infrared electric-field-driven scanning tunneling microscopy with a time resolution higher than 30 fs

Y Arashida, H Mogi, M Ishikawa, I Igarashi… - Acs …, 2022 - ACS Publications
Electric-field-driven scanning tunneling microscopy (STM) that uses carrier envelope phase-
controlled pulses in the THz region (THz-STM) has been attracting considerable attention …

Synthesis and direct sampling of single-cycle light transients by electron tunneling in a nanodevice

Y Luo, A Martin-Jimenez, F Neubrech, N Liu… - ACS …, 2023 - ACS Publications
The generation and direct time-domain sampling of ultrashort and ultra-broadband laser
pulses are at the forefront of time-resolved spectroscopy and attosecond science. Although …

Nanoscale coherent phonon spectroscopy

S Liu, A Hammud, I Hamada, M Wolf, M Müller… - Science …, 2022 - science.org
Coherent phonon spectroscopy can provide microscopic insight into ultrafast lattice
dynamics and its coupling to other degrees of freedom under nonequilibrium conditions …

Single-molecule photoelectron tunnelling spectroscopy

H Liu, L Chen, H Zhang, Z Yang, J Ye, P Zhou… - Nature Materials, 2023 - nature.com
Experimental mapping of transmission is essential for understanding and controlling charge
transport through molecular devices and materials. Here we developed a single-molecule …

All-optical subcycle microscopy on atomic length scales

T Siday, J Hayes, F Schiegl, F Sandner, P Menden… - Nature, 2024 - nature.com
Bringing optical microscopy to the shortest possible length and time scales has been a long-
sought goal, connecting nanoscopic elementary dynamics with the macroscopic …

Electrical manipulation of quantum coherence in a two-level molecular system

L Wang, D Bai, Y Xia, W Ho - Physical Review Letters, 2023 - APS
We report the manipulation of ultrafast quantum coherence of a two-level single hydrogen
molecular system by employing static electric field from the sample bias in a femtosecond …

Attosecond metrology of the two-dimensional charge distribution in molecules

V Loriot, A Boyer, S Nandi, CM González-Collado… - Nature Physics, 2024 - nature.com
Photoionization as a half-scattering process is not instantaneous. Usually, time delays in
photoionization are on the order of tens of attoseconds. In going from a single atom to a …