Massively parallel classical logic via coherent dynamics of an ensemble of quantum systems with dispersion in size

H Gattuso, RD Levine… - Proceedings of the …, 2020 - National Acad Sciences
Quantum parallelism can be implemented on a classical ensemble of discrete level quantum
systems. The nanosystems are not quite identical, and the ensemble represents their …

Coherent electronic and nuclear dynamics in a rhodamine heterodimer–DNA supramolecular complex

M Cipolloni, B Fresch, I Occhiuto, P Rukin… - Physical Chemistry …, 2017 - pubs.rsc.org
Elucidating the role of quantum coherences in energy migration within biological and
artificial multichromophoric antenna systems is the subject of an intense debate. It is also a …

Spectral shift, electronic coupling and exciton delocalization in nanocrystal dimers: insights from all-atom electronic structure computations

M Coden, P De Checchi, B Fresch - Nanoscale, 2020 - pubs.rsc.org
Delocalization of excitons promoted by electronic coupling between clusters or quantum
dots (QD) changes the dynamical processes in nanostructured aggregates enhancing …

Coherent exciton dynamics in ensembles of size-dispersed CdSe quantum dot dimers probed via ultrafast spectroscopy: A quantum computational study

H Gattuso, B Fresch, RD Levine, F Remacle - Applied Sciences, 2020 - mdpi.com
Featured Application Our results on the quantum electronic dynamics of quantum dots pave
the way to several applications in nanoscience. The large density of purely excitonic …

Effect of Different Conformational Distributions on the Ultrafast Coherence Dynamics in Porphyrin-Based Polymers

A Volpato, M Zerbetto, L Bolzonello… - The Journal of …, 2019 - ACS Publications
The optical and transport properties of biological and artificial multichromophoric functional
materials are strongly affected by the disorder and electron–vibration couplings. The …

A probabilistic finite state logic machine realized experimentally on a single dopant atom

B Fresch, J Bocquel, S Rogge, RD Levine… - Nano Letters, 2017 - ACS Publications
Exploiting the potential of nanoscale devices for logic processing requires the
implementation of computing functionalities departing from the conventional switching …

Implementation of Multivariable Logic Functions in Parallel by Electrically Addressing a Molecule of Three Dopants in Silicon

B Fresch, J Bocquel, D Hiluf, S Rogge… - …, 2017 - Wiley Online Library
To realize low‐power, compact logic circuits, one can explore parallel operation on single
nanoscale devices. An added incentive is to use multivalued (as distinct from Boolean) logic …

Multivalued logic at the nanoscale

B Fresch, MV Klymenko, RD Levine, F Remacle - Computational Matter, 2018 - Springer
Molecular and nanostructured systems for logic processing are typically characterized by
more than two internal states. The implementation of multivalued logic is thus a natural …

Implementation of Probabilistic Algorithms by Multi‐chromophoric Molecular Networks with Application to Multiple Travelling Pathways

B Fresch, F Remacle, RD Levine - ChemPhysChem, 2017 - Wiley Online Library
The implementation of probabilistic algorithms by deterministic hardware is demanding and
requires hundreds of instructions to generate a pseudo‐random sequence of numbers. On …

Computing by non-linear optical molecular response

B Fresch, TM Yan, D Hiluf, E Collini, RD Levine… - Computational …, 2018 - Springer
Non-linear optical spectroscopies probe the dynamics of optically active molecular systems
interacting with a sequence of laser pulses. By encoding logical inputs into the allowed …