Quantum information and algorithms for correlated quantum matter

K Head-Marsden, J Flick, CJ Ciccarino… - Chemical …, 2020 - ACS Publications
Discoveries in quantum materials, which are characterized by the strongly quantum-
mechanical nature of electrons and atoms, have revealed exotic properties that arise from …

Octacyanidometallates for multifunctional molecule-based materials

S Chorazy, JJ Zakrzewski, M Magott… - Chemical Society …, 2020 - pubs.rsc.org
Octacyanidometallates have been successfully employed in the design of heterometallic
coordination systems offering a spectacular range of desired physical properties with great …

The dynamic ligand field of a molecular qubit: decoherence through spin–phonon coupling

R Mirzoyan, RG Hadt - Physical Chemistry Chemical Physics, 2020 - pubs.rsc.org
Quantum coherence of S= 1/2 transition metal-based quantum bits (qubits) is strongly
influenced by the magnitude of spin–phonon coupling. While this coupling is recognized as …

Introduction of spin centers in single crystals of

M Sinha, TJ Pearson, TR Reeder, HK Vivanco… - Physical Review …, 2019 - APS
Developing the field of quantum information science (QIS) hinges upon designing viable
qubits, the smallest unit in quantum computing. One approach to creating qubits is …

Molecular-Engineered Biradicals Based on the YIII-Phthalocyanine Platform

N Suryadevara, AK Boudalis… - Journal of the …, 2023 - ACS Publications
A mixed-ligand phthalocyanine/porphyrin yttrium (III) radical double-decker complex (DD)
was synthesized using the custom-made 5, 10, 15-tris (4-methoxyphenyl)-20-(4 …

Enabling single qubit addressability in a molecular semiconductor comprising gold-supported organic radicals

J McGuire, HN Miras, E Richards, S Sproules - Chemical Science, 2019 - pubs.rsc.org
A bis (dithiolene) gold complex is presented as a model for an organic molecular electron
spin qubit attached to a metallic surface that acts as a conduit to electrically address the …

Impact of ligand chlorination and counterion tuning on high-field spin relaxation in a series of V (iv) complexes

R Martinez, CE Jackson, Ö Üngör, J van Tol… - Dalton …, 2023 - pubs.rsc.org
Methods of controlling spin coherence by molecular design are essential to efforts to
develop molecular qubits for quantum information and sensing applications. In this …

Electronic structure study of divanadium complexes with rigid covalent coordination: potential molecular qubits with slow spin relaxation

S Sproules - Dalton Transactions, 2021 - pubs.rsc.org
The electronic structures of homovalent [V2 (μ-S2) 2 (R2dtc) 4](R= Et, iBu) and mixed-valent
[V2 (μ-S2) 2 (R2dtc) 4]+ are reported here. The soft-donor, eight-coordinate ligand shell …

Synthesis and Characterization of 4d and 5d Cyanometallate Compounds for Molecular Magnetism

FJ Birk - 2019 - search.proquest.com
This research describes the synthesis and characterization of cyanometallate compounds
based on 4d and 5d transition metal ions. Since the discovery of [Mnv12 (CHv3COO) v16 …

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S Sproules - Transactions, 2017 - scholar.archive.org
The electronic structures of homovalent [V2 (μ-S2) 2 (R2dtc) 4](R= Et, iBu) and mixed-valent
[V2 (μ-S2) 2 (R2dtc) 4]+ are reported here. The soft-donor, eight-coordinate ligand shell …