Toward promising candidates of quantum information processing, the rapid development of
lanthanide-based single-molecule magnets (Ln-SMMs) highlights design strategies in …

Molecular magnetism, though distinctly a field within chemistry, encompasses much more
than synthesis and has strong links with other disciplines across the physical sciences …

Molecular spins are promising building blocks of future quantum technologies thanks to the
unparalleled flexibility provided by chemistry, which allows the design of complex structures …

Implementation of modern Quantum Technologies might benefit from the remarkable
quantum properties shown by molecular spin systems. In this Perspective, we highlight the …

The second quantum revolution hinges on the creation of materials that unite atomic
structural precision with electronic and structural tunability. A molecular approach to …

The study of how spin interacts with lattice vibrations and relaxes to equilibrium provides
unique insights into its chemical environment and the relation between electronic structure …

Vibronic coupling, the interaction between molecular vibrations and electronic states, is a
fundamental effect that profoundly affects chemical processes. In the case of molecular …

We perform a systematic investigation of the spin-phonon coupling leading to spin relaxation
in the prototypical mononuclear single molecule magnet [(tpaPh) Fe]−. In particular we …

Practical implementation of highly coherent molecular spin qubits for challenging
technological applications, such as quantum information processing or quantum sensing …

Over recent decades, much effort has been made to lengthen spin relaxation/decoherence
times of single-molecule magnets and molecular qubits by following different chemical …