Molecular spins for quantum computation

A Gaita-Ariño, F Luis, S Hill, E Coronado - Nature chemistry, 2019 - nature.com
Spins in solids or in molecules possess discrete energy levels, and the associated quantum
states can be tuned and coherently manipulated by means of external electromagnetic …

Single-molecule magnets beyond a single lanthanide ion: the art of coupling

YC Chen, ML Tong - Chemical Science, 2022 - pubs.rsc.org
The promising future of storing and processing quantized information at the molecular level
has been attracting the study of Single-Molecule Magnets (SMMs) for almost three decades …

The second quantum revolution: role and challenges of molecular chemistry

M Atzori, R Sessoli - Journal of the American Chemical Society, 2019 - ACS Publications
Implementation of modern Quantum Technologies might benefit from the remarkable
quantum properties shown by molecular spin systems. In this Perspective, we highlight the …

Rare-earth based tetrapyrrolic sandwiches: chemistry, materials and applications

AG Martynov, Y Horii, K Katoh, Y Bian, J Jiang… - Chemical Society …, 2022 - pubs.rsc.org
The unique properties of natural tetrapyrrolic compounds have inspired the rapid growth of
research interest in the design and synthesis of artificial porphyrinoids and their metal …

Molecular magnetism

NF Chilton - Annual Review of Materials Research, 2022 - annualreviews.org
Molecular magnetism, though distinctly a field within chemistry, encompasses much more
than synthesis and has strong links with other disciplines across the physical sciences …

Field-and temperature-dependent quantum tunnelling of the magnetisation in a large barrier single-molecule magnet

YS Ding, KX Yu, D Reta, F Ortu, REP Winpenny… - Nature …, 2018 - nature.com
Understanding quantum tunnelling of the magnetisation (QTM) in single-molecule magnets
(SMMs) is crucial for improving performance and achieving molecule-based information …

A perspective on scaling up quantum computation with molecular spins

S Carretta, D Zueco, A Chiesa, Á Gómez-León… - Applied Physics …, 2021 - pubs.aip.org
Artificial magnetic molecules can contribute to progressing toward large scale quantum
computation by (a) integrating multiple quantum resources and (b) reducing the …

High-temperature magnetic blocking in a monometallic dysprosium azafullerene single-molecule magnet

Z Hu, Y Wang, A Ullah, GM Gutiérrez-Finol… - Chem, 2023 - cell.com
Single-molecule magnets (SMMs) showing magnetic blocking near or above liquid nitrogen
temperature have recently been achieved by inducing exceptionally strong and axial crystal …

Low-coordinate mononuclear lanthanide complexes as molecular nanomagnets

AK Bar, P Kalita, MK Singh, G Rajaraman… - Coordination Chemistry …, 2018 - Elsevier
The discovery that some bis-(phthalocyaninato) lanthanide complexes are molecular
magnets triggered interest in lanthanide ion complexes. Theoretical and experimental …

A reaction-coordinate perspective of magnetic relaxation

CE Jackson, IP Moseley, R Martinez, S Sung… - Chemical Society …, 2021 - pubs.rsc.org
Understanding and utilizing the dynamic quantum properties of metal ions is the frontier of
many next generation technologies. One property in particular, magnetic relaxation, is a …