Helium spin echo experiments combined with ab initio based Langevin molecular dynamics simulations are used to quantify the adsorbate-substrate coupling during the thermal …
I Calvo-Almazán, P Fouquet - The European Physical Journal Special …, 2012 - Springer
Neutron scattering techniques such as quasi-elastic neutron scattering, QENS, have proven to be well-suited tools for studying structure and dynamics of surface adsorbed molecules. In …
I Calvo-Almazán, E Bahn, MM Koza, M Zbiri… - Carbon, 2014 - Elsevier
New insight into the nature of diffusion and the origin of friction of a prototype system for weak physisorption–benzene molecules, C 6 H 6, adsorbed on the basal plane (0 0 0 1) of …
Surface diffusion is described in terms of the intermediate scattering function in the time domain and reciprocal space. Two extreme time regimes are analyzed, ballistic (very short …
We present a combined experimental and theoretical study of the self-diffusion of ammonia on exfoliated graphite. Using neutron time-of-flight spectroscopy we are able to resolve the …
PSM Townsend, DJ Ward - Journal of Physics Communications, 2018 - iopscience.iop.org
We derive an analytical expression for the intermediate scattering function of a particle on a flat surface obeying the Generalised Langevin equation, with exponential memory friction …
Helium-3 surface spin echo spectroscopy (HeSE) has been used to measure the diffusive dynamics of adsorbates on close-packed metal surfaces, namely hydrogen on Cu (111), Pd …
The vibrational excitation of molecules adsorbed on a surface is typically probed by spectroscopic techniques such as infrared or Raman spectroscopy. In the present article we …
S Miret-Artés - Journal of Physics Communications, 2018 - iopscience.iop.org
Surface diffusion of small adsorbates is analyzed in terms of the so-called intermediate scattering function and dynamic structure factor, observables in experiments using the well …