Microrheology of colloidal systems

AM Puertas, T Voigtmann - Journal of Physics: Condensed …, 2014 - iopscience.iop.org
Microrheology was proposed almost twenty years ago as a technique to obtain rheological
properties in soft matter from the microscopic motion of colloidal tracers used as probes …

Dynamics of self-propelled Janus particles in viscoelastic fluids

JR Gomez-Solano, A Blokhuis, C Bechinger - Physical review letters, 2016 - APS
We experimentally investigate active motion of spherical Janus colloidal particles in a
viscoelastic fluid. Self-propulsion is achieved by a local concentration gradient of a critical …

Memory-induced transition from a persistent random walk to circular motion for achiral microswimmers

N Narinder, C Bechinger, JR Gomez-Solano - Physical review letters, 2018 - APS
We experimentally study the motion of light-activated colloidal microswimmers in a
viscoelastic fluid. We find that, in such a non-Newtonian environment, the active colloids …

Differential dynamic microscopy microrheology of soft materials: A tracking-free determination of the frequency-dependent loss and storage moduli

P Edera, D Bergamini, V Trappe, F Giavazzi… - Physical Review …, 2017 - APS
Particle-tracking microrheology (PT-μ r) exploits the thermal motion of embedded particles to
probe the local mechanical properties of soft materials. Despite its appealing conceptual …

Burst-by-burst measurement of rotational diffusion at nanosecond resolution reveals hot-brownian motion and single-chain binding

N Asgari, MD Baaske, M Orrit - ACS nano, 2023 - ACS Publications
We record dark-field scattering bursts of individual gold nanorods, 52× 15 nm2 in average
size, freely diffusing in water suspension. We deduce their Brownian rotational diffusion …

Measuring translational, rotational, and vibrational dynamics in colloids with digital holographic microscopy

J Fung, KE Martin, RW Perry, DM Kaz, R McGorty… - Optics express, 2011 - opg.optica.org
We discuss a new method for simultaneously probing translational, rotational, and
vibrational dynamics in dilute colloidal suspensions using digital holographic microscopy …

Nanoscale rheology and anisotropic diffusion using single gold nanorod probes

M Molaei, E Atefi, JC Crocker - Physical review letters, 2018 - APS
The complex rotational and translational Brownian motion of anisotropic particles depends
on their shape and the viscoelasticity of their surroundings. Because of their strong optical …

Picoliter viscometry using optically rotated particles

SJ Parkin, G Knöner, TA Nieminen… - Physical Review E …, 2007 - APS
Important aspects in the field of microrheology are studies of the viscosity of fluids within
structures with micrometer dimensions and fluid samples where only microliter volumes are …

Rotational analysis of spherical, optically anisotropic janus particles by dynamic microscopy

A Wittmeier, A Leeth Holterhoff, J Johnson, JG Gibbs - Langmuir, 2015 - ACS Publications
We analyze the rotational dynamics of spherical colloidal Janus particles made from silica
(SiO2) with a hemispherical gold/palladium (Au/Pd) cap. Since the refractive index …

Direct observation of spatiotemporal heterogeneous gelation by rotational tracking of a single anisotropic nanoprobe

H Sun, Z Wang, Y He - Acs Nano, 2019 - ACS Publications
Polymer network gels usually exhibit spatial heterogeneity of local defects and cross-link
density, which can affect their elasticity on the microscopic scale differently. The ability to …