Luminescent Organic Triplet Diradicals as Optically Addressable Molecular Qubits

SM Kopp, S Nakamura, BT Phelan… - Journal of the …, 2024 - ACS Publications
Optical-spin interfaces that enable the photoinitialization, coherent microwave manipulation,
and optical read-out of ground state spins have been studied extensively in solid-state …

Singlet–Triplet Inversion in Triangular Boron Carbon Nitrides

M Bedogni, F Di Maiolo - Journal of Chemical Theory and …, 2024 - ACS Publications
The discovery of singlet–triplet (ST) inversion in some π-conjugated triangle-shaped boron
carbon nitrides is a remarkable breakthrough that defies Hund's first rule. Deeply rooted in …

Turning on Organic Radical Emitters

M Dubbini, F Bonvini, L Savi… - The Journal of Physical …, 2024 - ACS Publications
Radical emitters have attracted considerable interest because of their potential to surpass
the limitations of singlet emitters due to spin statistics, thereby revolutionizing organic LEDs …

Enhancing the Optically Detected Magnetic Resonance Signal of Organic Molecular Qubits

YR Poh, J Yuen-Zhou - ACS Central Science, 2025 - ACS Publications
In quantum information science and sensing, electron spins are often purified into a specific
polarization through an optical-spin interface, a process known as optically detected …

Emission enhancement in a luminescent polychlorinated diphenylpyridylmethyl radical through coordination to silver (I)

T Mibu, R Matsuoka, M Nagasaka, T Kusamoto - Dalton Transactions, 2025 - pubs.rsc.org
A luminescent silver (I) complex containing a luminescent radical ligand was prepared for
the first time. Coordination to AgI enhanced and red-shifted the radical-centered emission …

Enhancing the ODMR Signal of Organic Molecular Qubits

YR Poh, J Yuen-Zhou - arXiv preprint arXiv:2409.19249, 2024 - arxiv.org
In the fields of quantum information science and sensing, electron spins are often purified
into a specific polarisation through an optical-spin interface, a process known as optically …

[HTML][HTML] Ultrafast Excited State Dynamics of a Verdazyl Diradical System

C Clark, F Pawłowski, DJR Brook, C Grieco - Photochem, 2024 - mdpi.com
While the photophysics of closed-shell organic molecules is well established, much less is
known about open-shell systems containing interacting radical pairs. In this work, we …

Optical read and write of spin states in organic diradicals

R Chowdhury, P Murto, NA Panjwani, Y Sun… - arXiv preprint arXiv …, 2024 - arxiv.org
Optical control and read-out of the ground state spin structure has been demonstrated for
defect states in crystalline semiconductors, including the diamond NV-center, and these are …

Stable Luminescent Diradicals: The Emergence and Potential Applications

Y Zhu, Z Zhu, S Wang, Q Peng… - Angewandte Chemie … - Wiley Online Library
Stable luminescent diradicals, characterized by the presence of two unpaired electrons,
exhibit unique photophysical properties that are sensitive to external stimuli such as …