Multiscale CO2 Electrocatalysis to C2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication

T Yan, X Chen, L Kumari, J Lin, M Li, Q Fan… - Chemical …, 2023 - ACS Publications
Electrosynthesis of value-added chemicals, directly from CO2, could foster achievement of
carbon neutral through an alternative electrical approach to the energy-intensive …

Stability Issues in Electrochemical CO2 Reduction: Recent Advances in Fundamental Understanding and Design Strategies

W Lai, Y Qiao, Y Wang, H Huang - Advanced Materials, 2023 - Wiley Online Library
Electrochemical CO2 reduction reaction (CO2RR) offers a promising approach to close the
anthropogenic carbon cycle and store intermittent renewable energy in fuels or chemicals …

Coverage-driven selectivity switch from ethylene to acetate in high-rate CO2/CO electrolysis

P Wei, D Gao, T Liu, H Li, J Sang, C Wang… - Nature …, 2023 - nature.com
Tuning catalyst microenvironments by electrolytes and organic modifications is effective in
improving CO2 electrolysis performance. An alternative way is to use mixed CO/CO2 feeds …

Surface passivation for highly active, selective, stable, and scalable CO2 electroreduction

J Zhu, J Li, R Lu, R Yu, S Zhao, C Li, L Lv, L Xia… - Nature …, 2023 - nature.com
Electrochemical conversion of CO2 to formic acid using Bismuth catalysts is one the most
promising pathways for industrialization. However, it is still difficult to achieve high formic …

Tailoring acidic microenvironments for carbon-efficient CO 2 electrolysis over a Ni–N–C catalyst in a membrane electrode assembly electrolyzer

H Li, H Li, P Wei, Y Wang, Y Zang, D Gao… - Energy & …, 2023 - pubs.rsc.org
CO2 electrolysis converting CO2 into valuable fuels and chemicals powered by renewable
electricity shows great promise for practical applications. However, it suffers from low energy …

Construction of C–N bonds from small-molecule precursors through heterogeneous electrocatalysis

J Li, Y Zhang, K Kuruvinashetti… - Nature Reviews Chemistry, 2022 - nature.com
Energy-intensive thermochemical processes within chemical manufacturing are a major
contributor to global CO2 emissions. With the increasing push for sustainability, the scientific …

Imidazolium-functionalized Mo3P nanoparticles with an ionomer coating for electrocatalytic reduction of CO2 to propane

M Esmaeilirad, Z Jiang, AM Harzandi, A Kondori… - Nature Energy, 2023 - nature.com
Propane is a tri-carbon (C3) alkane widely used as a fuel. Despite recent advances in CO2
electrocatalysis, the production of C3+ molecules directly from CO2 is challenging due to …

Carbon-efficient carbon dioxide electrolysers

A Ozden, FP García de Arquer, JE Huang, J Wicks… - Nature …, 2022 - nature.com
The electroreduction of CO2 (CO2R) is the conversion of CO2 to renewable fuels and
feedstocks, a promising technology that could support the transition from fossil to renewable …

Energy- and carbon-efficient CO2/CO electrolysis to multicarbon products via asymmetric ion migration–adsorption

A Ozden, J Li, S Kandambeth, XY Li, S Liu, O Shekhah… - Nature Energy, 2023 - nature.com
Abstract Carbon dioxide/monoxide (CO2/CO) electrolysis provides a means to convert
emissions into multicarbon products. However, impractical energy and carbon efficiencies …

Bifunctional ionomers for efficient co-electrolysis of CO2 and pure water towards ethylene production at industrial-scale current densities

W Li, Z Yin, Z Gao, G Wang, Z Li, F Wei, X Wei, H Peng… - Nature Energy, 2022 - nature.com
Many CO2 electrolysers under development use liquid electrolytes (KOH solutions, for
example), yet using solid-state polymer electrolytes can in principle improve efficiency and …